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2009


Full phase and amplitude control in computer-generated holography
Full phase and amplitude control in computer-generated holography

Fratz, M., Fischer, P., Giel, D. M.

OPTICS LETTERS, 34(23):3659-3661, 2009 (article)

Abstract
We report what we believe to be the first realization of a computer-generated complex-valued hologram recorded in a single film of photoactive polymer. Complex-valued holograms give rise to a diffracted optical field with control over its amplitude and phase. The holograms are generated by a one-step direct laser writing process in which a spatial light modulator (SLM) is imaged onto a polymer film. Temporal modulation of the SLM during exposure controls both the strength of the induced birefringence and the orientation of the fast axis. We demonstrate that complex holograms can be used to impart arbitrary amplitude and phase profiles onto a beam and thereby open new possibilities in the control of optical beams. (C) 2009 Optical Society of America

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2009


[BibTex]


Digital polarization holograms with defined magnitude and orientation of each pixel's birefringence
Digital polarization holograms with defined magnitude and orientation of each pixel’s birefringence

Fratz, M., Giel, D. M., Fischer, P.

OPTICS LETTERS, 34(8):1270-1272, 2009 (article)

Abstract
A new form of digital polarization holography is demonstrated that permits both the amplitude and the phase of a diffracted beam to be independently controlled. This permits two independent intensity images to be stored in the same hologram. To fabricate the holograms, a birefringence with defined retardance and orientation of the fast axis is recorded into a photopolymer film. The holograms are selectively read out by choosing the polarization state of the read beam. Polarization holograms of this kind increase the data density in holographic data storage and allow higher quality diffractive optical elements to be written. (C) 2009 Optical Society of America

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Controlled Propulsion of Artificial Magnetic Nanostructured Propellers
Controlled Propulsion of Artificial Magnetic Nanostructured Propellers

Ghosh, A., Fischer, P.

NANO LETTERS, 9(6):2243-2245, 2009, Featured highlight ‘Nanotechnology: The helix that delivers’ Nature 459, 13 (2009). (article)

Abstract
For biomedical applications, such as targeted drug delivery and microsurgery, it is essential to develop a system of swimmers that can be propelled wirelessly in fluidic environments with good control. Here, we report the construction and operation of chiral colloidal propellers that can be navigated in water with micrometer-level precision using homogeneous magnetic fields. The propellers are made via nanostructured surfaces and can be produced in large numbers. The nanopropellers can carry chemicals, push loads, and act as local probes in rheological measurements.

Featured highlight ‘Nanotechnology: The helix that delivers’ Nature 459, 13 (2009).

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Video - Nanospropellers DOI [BibTex]

Video - Nanospropellers DOI [BibTex]


Absolute Asymmetric Reduction Based on the Relative Orientation of Achiral Reactants
Absolute Asymmetric Reduction Based on the Relative Orientation of Achiral Reactants

Kuhn, A., Fischer, P.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 48(37):6857-6860, 2009 (article)

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One-dimensional phthalocyanine nanostructures directed by gold templates

Krauss, T. N., Barrena, E., Lohmüller, T., Kelsch, M., Breitling, A., Van Aken, P. A., Spatz, J., Dosch, H.

{Chemistry of Materials}, 21, pages: 5010-5015, 2009 (article)

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Near-edge X-ray absorption fine-structure microscopy of organic and magnetic materials

Ade, H., Stoll, H.

{Nature Materials}, 8, pages: 281-290, 2009 (article)

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X-ray imaging of the dynamic magnetic vortex core deformation

Vansteenkiste, A., Chou, K. W., Weigand, M., Curcic, M., Sackmann, V., Stoll, H., Tyliszczak, T., Woltersdorf, G., Back, C. H., Schütz, G., Van Waeyenberge, B.

{Nature Physics}, 5, pages: 332-334, 2009 (article)

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Order\textendashdisorder transition and valence state of ytterbium in YbAuxGa2-x(0.26 \textless\textequalsx \textless\textequals1.31)

Gumeniuk, R., Bischoff, E., Burkhardt, U., Prots, Y., Schnelle, W., Vasylechko, L., Schmidt, M., Kuzma, Y., Grin, Y.

{Journal of Solid State Chemistry}, 182(12):3374-3382, 2009 (article)

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Coercivity of ledge-type L10-FePt/Fe nanocomposites with perpendicular magnetization

Goll, D., Breitling, A.

{Applied Physics Letters}, 94, 2009 (article)

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Time-resolved X-ray microscopy of nanoparticle aggregates under oscillatory shear

Auernhammer, G. K., Fauth, K., Ullrich, B., Zhao, J., Weigand, M., Vollmer, D.

{Journal of Synchrotron Radiation}, 16, pages: 307-309, 2009 (article)

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Micromagnetism of advanced hard magnetic materials

Kronmüller, H., Goll, D.

{International Journal of Materials Research}, 100, pages: 640-651, 2009 (article)

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Confinement of MgH2 nanoclusters within nanoporous aerogel scaffold materials

Nielsen, T. K., Manickam, K., Hirscher, M., Besenbacher, F., Jensen, T. R.

{American Chemical Society Nano}, 3(11):3521-3528, 2009 (article)

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Possible definition of atom- and bond-resolved contributions to the magnetocrystalline anisotropy energy

Subkow, S., Fähnle, M.

{Physical Review B}, 80, 2009 (article)

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Complex magnetic phase in submonolayer Fe stripes on Pt(977)

Honolka, J., Lee, T. Y., Kuhnke, K., Repetto, D., Sessi, V., Wahl, P., Buchsbaum, A., Varga, P., Gardonio, S., Carbone, C., Krishnakumar, S. R., Gambardella, P., Komelj, M., Singer, R., Fähnle, M., Fauth, K., Schütz, G., Enders, A., Kern, K.

{Physical Review B}, 79, 2009 (article)

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Local and nonlocal atomic contributions to unit-cell damping in near-adiabatic collinear magnetization dynamics

Seib, J., Steiauf, D., Fähnle, M.

{Physical Review B}, 79, 2009 (article)

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Temperature-dependent critical currents in superconducting YBa2Cu3O7-δand ferromagnetic La2/3Ca1/3MnO3 hybrid structures

Djupmyr, M., Soltan, S., Habermeier, H.-U., Albrecht, J.

{Physical Review B}, 80, 2009 (article)

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High surface area polyHIPEs with hierarchical pore system

Schwab, M. G., Senkovska, I., Rose, M., Klein, N., Koch, M., Pahnke, J., Jonschker, G., Schmitz, B., Hirscher, M., Kaskel, S.

{Soft Matter}, 5, pages: 1055-1059, 2009 (article)

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Grain boundary wetting phase transformations in the Zn-Sn and Zn-In systems

Gornakova, A. S., Straumal, B. B., Tsurekawa, S., Chang, L.-S., Nekrasov, A. N.

{Reviews on Advanced Materials Science}, 21(1):18-26, 2009 (article)

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Magnetization study of nanograined pure and Mn-doped ZnO films: formation of a ferromagnetic grain-boundary foam

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Myatiev, A. A., Straumal, P. B., Schütz, G., van Aken, P. A., Goering, E., Baretzky, B.

{Physical Review B}, 79, 2009 (article)

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In situ synthesis and hydrogen storage properties of PdNi alloy nanoparticles in an ordered mesoporous carbon template

Campesi, R., Cuevas, F., Leroy, E., Hirscher, M., Gadiou, R., Vix-Guterl, C., Latroche, M.

{Microporous and Mesoporous Materials}, 117, pages: 511-514, 2009 (article)

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Mit Röntgenblitzen zu neuen Erkenntnissen

Hedderich, R., Weigand, M., Baretzky, B.

{Nanotechnik - Molek\"ule Materialien Mikrosysteme}, (6 (Beilage zu Photonik 41. 2009)), 2009 (article)

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Second-order faceting-roughening of the tilt grain boundary in zinc

Straumal, B. B., Gornakova, A. S., Sursaeva, V. G., Yashnikov, V. P.

{International Journal of Materials Research}, 100(4):525-529, 2009 (article)

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Improvement of interface structure and magnetic properties of Co on Si (100) by surfactant (Sb) mediated growth

Dash, S. P., Goll, D., Carstanjen, H. D.

{Applied Physics A}, 97(3):651-656, 2009 (article)

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Effect of severe plastic deformation on the coercivity of Co-Cu alloys

Straumal, B. B., Protasova, S. G., Mazilkin, A. A., Baretzky, B., Goll, D., Gunderov, D. V., Valiev, R. Z.

{Philosophical Magazine Letters}, 89(10):649-654, 2009 (article)

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Magnetic properties of cobalt-covered MgB2 films

Treiber, S., Stuhlhofer, B., Habermeier, H.-U., Albrecht, J.

{Superconductor Science and Technology}, 22, 2009 (article)

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Reconstruction of historic alloys for pipe organs brings true Baroque music back to life

Baretzky, B., Friesel, M., Straumal, B.

{Japan Organist}, 36, pages: 29-38, 2009 (article)

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Exchange-coupled L10-FePt/Fe composite patterns with perpendicular magnetization

Breitling, A., Bublat, T., Goll, D.

{Physica Status Solidi - Rapid Research Letters}, 3(5):130-132, 2009 (article)

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Proton NMR studies of the NaAlH4 structure

Valiente-Banuet, L. E., Majer, G., Müller, K.

{Journal of Magnetic Resonance}, 200, pages: 280-284, 2009 (article)

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Magnetism of FePt surface alloys

Honolka, J., Lee, T. Y., Kuhnke, K., Enders, A., Skomski, R., Bornemann, S., Mankovsky, S., Minár, J., Staunton, J., Ebert, H., Hessler, M., Fauth, K., Schütz, G., Buchsbaum, A., Schmid, M., Varga, P., Kern, K.

{Physical Review Letters}, 102(6), 2009 (article)

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Enhanced 95Zr diffusion in grain boundaries of nano-crystalline ZrO2 \mbox⋅ 9.5 mol\textpercent Y2O3

Drings, H., Brossmann, U., Carstanjen, H. D., Szökefalvi-Nagy, A., Noll, C., Schaefer, H.-E.

{Physica Status Solidi (A)}, 206(1):54-58, 2009 (article)

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Magnetism of nanostructured materials for advanced magnetic recording

Goll, D.

{International Journal of Materials Research}, 100, pages: 652-662, 2009 (article)

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Vortex core switching by coherent excitation with single in-plane magnetic field pulses

Weigand, M., van Waeyenberge, B., Vansteenkiste, A., Curcic, M., Sackmann, V., Stoll, H., Tyliszczak, T., Kaznatcheev, K., Bertwistle, D., Woltersdorf, G., Back, C. H., Schütz, G.

{Physical Review Letters}, 102, 2009 (article)

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Increase of Mn solubility with decreasing grain size in ZnO

Straumal, B., Baretzky, B., Mazilkin, A., Protasova, S., Myatiev, A., Straumal, P.

{Journal of the European Ceramic Society}, 29(10):1963-1970, 2009 (article)

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Fe-C nanograined alloys obtained by high-pressure torsion: Structure and magnetic properties

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Dobatkin, S. V., Rodin, A. O., Baretzky, B., Goll, D., Schütz, G.

{Materials Science and Engineering A}, 503, pages: 185-189, 2009 (article)

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Chiral symmetry breaking of magnetic vortices by sample roughness

Vansteenkiste, A., Weigand, M., Curcic, M., Stoll, H., Schütz, G., Van Waeyenberge, B.

{New Journal of Physics}, 11, 2009 (article)

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Extended s-d model for magnetization dynamics of strongly noncollinear configurations

De Angeli, L., Steiauf, D., Singer, R., Köberle, I., Dietermann, F., Fähnle, M.

{Physical Review B}, 79, 2009 (article)

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Superconducting phase formation in random neck syntheses: a study of the Y-Ba-Cu-O system by magneto-optics and magnetometry

Willems, J. B., Albrecht, J., Landau, I. L., Hulliger, J.

{Superconductor Science and Technology}, 22, 2009 (article)

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Determination of spin moments from magnetic EXAFS

Popescu, V., Gü\ssmann, M., Fähnle, M., Schütz, G.

{Physical Review B}, 79, 2009 (article)

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Linewidth of ferromagnetic resonance for systems with anisotropic damping

Seib, J., Steiauf, D., Fähnle, M.

{Physical Review B}, 79, 2009 (article)

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Structural and magnetic deconvolution of FePt/FeOx-nanoparticles using x-ray magnetic circular dichroism

Nolle, D., Goering, E., Tietze, T., Schütz, G., Figuerola, A., Manna, L.

{New Journal of Physics}, 11, 2009 (article)

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Magnetic imaging with femtosecond temporal resolution

Li, J., Lee, M.-S., He, W., Redeker, B., Remhof, A., Amaladass, E., Hassel, C., Eimüller, T.

{Review of Scientific Instruments}, 80(7), 2009 (article)

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Elliott-Yafet mechanism and the discussion of femtosecond magnetization dynamics

Steiauf, D., Fähnle, M.

{Physical Review B}, 79, 2009 (article)

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Investigation of the stability of Mn12 single molecule magnets

Voss, S., Fonin, M., Burova, L., Burgert, M., Dedkov, Y. S., Preobrajenski, A. B., Goering, E., Groth, U., Kaul, A. R., Ruediger, U.

{Applied Physics A}, 94(3):491-495, 2009 (article)

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2006


Chiral molecules split light: Reflection and refraction in a chiral liquid
Chiral molecules split light: Reflection and refraction in a chiral liquid

Ghosh, A., Fischer, P.

PHYSICAL REVIEW LETTERS, 97(17), 2006, Featured highlight ‘Fundamental optical physics: Refraction’ Nature Photonics, Nov. 2006. (article)

Abstract
A light beam changes direction as it enters a liquid at an angle from another medium, such as air. Should the liquid contain molecules that lack mirror symmetry, then it has been predicted by Fresnel that the light beam will not only change direction, but will actually split into two separate beams with a small difference in the respective angles of refraction. Here we report the observation of this phenomenon. We also demonstrate that the angle of reflection does not equal the angle of incidence in a chiral medium. Unlike conventional optical rotation, which depends on the path-length through the sample, the reported reflection and refraction phenomena arise within a few wavelengths at the interface and thereby suggest a new approach to polarimetry that can be used in microfluidic volumes.

Featured highlight ‘Fundamental optical physics: Refraction’ Nature Photonics, Nov. 2006.

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2006


DOI [BibTex]


Direct chiral discrimination in NMR spectroscopy
Direct chiral discrimination in NMR spectroscopy

Buckingham, A., Fischer, P.

CHEMICAL PHYSICS, 324(1):111-116, 2006 (article)

Abstract
Conventional nuclear magnetic resonance spectroscopy is unable to distinguish between the two mirror-image forms (enantiomers) of a chiral molecule. This is because the NMR spectrum is determined by the chemical shifts and spin-spin coupling constants which - in the absence of a chiral solvent - are identical for the two enantiomers. We discuss how chirality may nevertheless be directly detected in liquid-state NMR spectroscopy: In a chiral molecule, the rotating nuclear magnetic moment induces an electric dipole moment in the direction perpendicular to itself and to the permanent magnetic field of the spectrometer. We present computations of the precessing electric polarization following a pi/2 pulse. Our estimates indicate that the electric polarization should be detectable in favourable cases. We also predict that application of an electrostatic field induces a chirally sensitive magnetization oscillating in the direction of the permanent magnetic field. We show that the electric-field-perturbed chemical shift tensor, the nuclear magnetic shielding polarizability, underlies these chiral NMR effects. (c) 2005 Elsevier B.V. All rights reserved.

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Ring-resonator-based frequency-domain optical activity measurements of a chiral liquid
Ring-resonator-based frequency-domain optical activity measurements of a chiral liquid

Vollmer, F., Fischer, P.

OPTICS LETTERS, 31(4):453-455, 2006 (article)

Abstract
Chiral liquids rotate the plane of polarization of linearly polarized light and are therefore optically active. Here we show that optical rotation can be observed in the frequency domain. A chiral liquid introduced in a fiber-loop ring resonator that supports left and right circularly polarized modes gives rise to relative frequency shifts that are a direct measure of the liquid's circular birefringence and hence of its optical activity. The effect is in principle not diminished if the circumference of the ring is reduced. The technique is similarly applicable to refractive index and linear birefringence measurements. (c) 2006 Optical Society of America.

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Sign of the refractive index in a gain medium with negative permittivity and permeability
Sign of the refractive index in a gain medium with negative permittivity and permeability

Chen, Y., Fischer, P., Wise, F.

JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 23(1):45-50, 2006 (article)

Abstract
We show how the sign of the refractive index in any medium may be derived using a rigorous analysis based on Einstein causality. In particular, we consider left-handed materials, i.e., media that have negative permittivities and permeabilities at the frequency of interest. We find that the consideration of gain in such media can give rise to a positive refractive index. (c) 2006 Optical Society of America.

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Influence of the substrate on the magnetic anisotropy of monatomic wires

Komelj, M., Steiauf, D., Fähnle, M.

{Physical Review B}, 73, 2006 (article)

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Mechanical properties of single-walled carbon nanotubes based on higher order Cauchy-Born rule

Guo, X., Wang, J. B., Zhang, H. W.

{International Journal of Solids and Structures}, 43, pages: 1276-1290, 2006 (article)

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