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2015


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Enzymatically active biomimetic micropropellers for the penetration of mucin gels

Walker (Schamel), D., Käsdorf, B. T., Jeong, H. H., Lieleg, O., Fischer, P.

Science Advances, 1(11):e1500501, December 2015 (article)

Abstract
In the body, mucus provides an important defense mechanism by limiting the penetration of pathogens. It is therefore also a major obstacle for the efficient delivery of particle-based drug carriers. The acidic stomach lining in particular is difficult to overcome because mucin glycoproteins form viscoelastic gels under acidic conditions. The bacterium Helicobacter pylori has developed a strategy to overcome the mucus barrier by producing the enzyme urease, which locally raises the pH and consequently liquefies the mucus. This allows the bacteria to swim through mucus and to reach the epithelial surface. We present an artificial system of reactive magnetic micropropellers that mimic this strategy to move through gastric mucin gels by making use of surface-immobilized urease. The results demonstrate the validity of this biomimetic approach to penetrate biological gels, and show that externally propelled microstructures can actively and reversibly manipulate the physical state of their surroundings, suggesting that such particles could potentially penetrate native mucus.

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link (url) DOI [BibTex]

2015


link (url) DOI [BibTex]


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The EChemPen: A Guiding Hand To Learn Electrochemical Surface Modifications

Valetaud, M., Loget, G., Roche, J., Hueken, N., Fattah, Z., Badets, V., Fontaine, O., Zigah, D.

J. of Chem. Ed., 92(10):1700-1704, September 2015 (article)

Abstract
The Electrochemical Pen (EChemPen) was developed as an attractive tool for learning electrochemistry. The fabrication, principle, and operation of the EChemPen are simple and can be easily performed by students in practical classes. It is based on a regular fountain pen principle, where the electrolytic solution is dispensed at a tip to locally modify a conductive surface by triggering a localized electrochemical reaction. Three simple model reactions were chosen to demonstrate the versatility of the EChemPen for teaching various electrochemical processes. We describe first the reversible writing/erasing of metal letters, then the electrodeposition of a black conducting polymer "ink", and finally the colorful writings that can be generated by titanium anodization and that can be controlled by the applied potential. These entertaining and didactic experiments are adapted for teaching undergraduate students that start to study electrochemistry by means of surface modification reactions.

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DOI [BibTex]

DOI [BibTex]


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3D-printed Soft Microrobot for Swimming in Biological Fluids

Qiu, T., Palagi, S., Fischer, P.

In Conf. Proc. IEEE Eng. Med. Biol. Soc., pages: 4922-4925, August 2015 (inproceedings)

Abstract
Microscopic artificial swimmers hold the potential to enable novel non-invasive medical procedures. In order to ease their translation towards real biomedical applications, simpler designs as well as cheaper yet more reliable materials and fabrication processes should be adopted, provided that the functionality of the microrobots can be kept. A simple single-hinge design could already enable microswimming in non-Newtonian fluids, which most bodily fluids are. Here, we address the fabrication of such single-hinge microrobots with a 3D-printed soft material. Firstly, a finite element model is developed to investigate the deformability of the 3D-printed microstructure under typical values of the actuating magnetic fields. Then the microstructures are fabricated by direct 3D-printing of a soft material and their swimming performances are evaluated. The speeds achieved with the 3D-printed microrobots are comparable to those obtained in previous work with complex fabrication procedures, thus showing great promise for 3D-printed microrobots to be operated in biological fluids.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Optimal Length of Low Reynolds Number Nanopropellers

Walker (Schamel), D., Kuebler, M., Morozov, K. I., Fischer, P., Leshansky, A. M.

Nano Letters, 15(7):4412-4416, June 2015 (article)

Abstract
Locomotion in fluids at the nanoscale is dominated by viscous drag. One efficient propulsion scheme is to use a weak rotating magnetic field that drives a chiral object. Froth bacterial flagella to artificial drills, the corkscrew is a universally useful chiral shape for propulsion in viscous environments. Externally powered magnetic micro- and nanomotors have been recently developed that allow for precise fuel-free propulsion in complex media. Here, we combine analytical and numerical theory with experiments on nanostructured screw-propellers to show that the optimal length is surprisingly short only about one helical turn, which is shorter than most of the structures in use to date. The results have important implications for the design of artificial actuated nano- and micropropellers and can dramatically reduce fabrication times, while ensuring optimal performance.

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DOI [BibTex]

DOI [BibTex]


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A theoretical study of potentially observable chirality-sensitive NMR effects in molecules

Garbacz, P., Cukras, J., Jaszunski, M.

Phys. Chem. Chem. Phys., 17(35):22642-22651, May 2015 (article)

Abstract
Two recently predicted nuclear magnetic resonance effects, the chirality-induced rotating electric polarization and the oscillating magnetization, are examined for several experimentally available chiral molecules. We discuss in detail the requirements for experimental detection of chirality-sensitive NMR effects of the studied molecules. These requirements are related to two parameters: the shielding polarizability and the antisymmetric part of the nuclear magnetic shielding tensor. The dominant second contribution has been computed for small molecules at the coupled cluster and density functional theory levels. It was found that DFT calculations using the KT2 functional and the aug-cc-pCVTZ basis set adequately reproduce the CCSD(T) values obtained with the same basis set. The largest values of parameters, thus most promising from the experimental point of view, were obtained for the fluorine nuclei in 1,3-difluorocyclopropene and 1,3-diphenyl-2-fluoro-3-trifluoromethylcyclopropene.

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DOI [BibTex]

DOI [BibTex]


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Dynamic Inclusion Complexes of Metal Nanoparticles Inside Nanocups

Alarcon-Correa, M., Lee, T. C., Fischer, P.

Angew. Chem. Int. Ed., 54(23):6730-6734, May 2015, Featured cover article. (article)

Abstract
Host-guest inclusion complexes are abundant in molecular systems and of fundamental importance in living organisms. Realizing a colloidal analogue of a molecular dynamic inclusion complex is challenging because inorganic nanoparticles (NPs) with a well-defined cavity and portal are difficult to synthesize in high yield and with good structural fidelity. Herein, a generic strategy towards the fabrication of dynamic 1: 1 inclusion complexes of metal nanoparticles inside oxide nanocups with high yield (> 70%) and regiospecificity (> 90%) by means of a reactive double Janus nanoparticle intermediate is reported. Experimental evidence confirms that the inclusion complexes are formed by a kinetically controlled mechanism involving a delicate interplay between bipolar galvanic corrosion and alloying-dealloying oxidation. Release of the NP guest from the nanocups can be efficiently triggered by an external stimulus. Featured cover article.

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DOI [BibTex]

DOI [BibTex]


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Surface roughness-induced speed increase for active Janus micromotors

Choudhury, U., Soler, L., Gibbs, J. G., Sanchez, S., Fischer, P.

Chem. Comm., 51(41):8660-8663, April 2015 (article)

Abstract
We demonstrate a simple physical fabrication method to control surface roughness of Janus micromotors and fabricate self-propelled active Janus microparticles with rough catalytic platinum surfaces that show a four-fold increase in their propulsion speed compared to conventional Janus particles coated with a smooth Pt layer.

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DOI [BibTex]

DOI [BibTex]


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Active colloidal microdrills

Gibbs, J. G., Fischer, P.

Chem. Comm., 51(20):4192-4195, Febuary 2015 (article)

Abstract
We demonstrate a chemically driven, autonomous catalytic microdrill. An asymmetric distribution of catalyst causes the helical swimmer to twist while it undergoes directed propulsion. A driving torque and hydrodynamic coupling between translation and rotation at low Reynolds number leads to drill-like swimming behaviour.

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DOI [BibTex]

DOI [BibTex]


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Selectable Nanopattern Arrays for Nanolithographic Imprint and Etch-Mask Applications

Jeong, H. H., Mark, A. G., Lee, T., Son, K., Chen, W., Alarcon-Correa, M., Kim, I., Schütz, G., Fischer, P.

Adv. Science, 2(7):1500016, 2015, Featured cover article. (article)

Abstract
A parallel nanolithographic patterning method is presented that can be used to obtain arrays of multifunctional nanoparticles. These patterns can simply be converted into a variety of secondary nanopatterns that are useful for nanolithographic imprint, plasmonic, and etch-mask applications.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


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Strukturelle und spektroskopische Eigenschaften epitaktischer FeMn/Co Exchange-Bias-Systeme

Schmidt, M.

Universität Stuttgart, Stuttgart, 2015 (phdthesis)

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link (url) DOI [BibTex]


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Fabrication and X-ray testing of true kinoform lenses with high efficiencies

Keskinbora, K., Sanli, U., Grévent, C., Schütz, G.

{Proceedings of SPIE}, 9592, SPIE, Bellingham, Washington, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Ultraschnelles Vortexkernschalten

Noske, M.

Universität Stuttgart, Stuttgart (und Cuvillier Verlag, Göttingen), 2015 (phdthesis)

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[BibTex]

[BibTex]


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Time-resolved imaging of pulse-induced magnetization reversal with a microwave assist field

Rao, S., Rhensius, J., Bisig, A., Mawass, M.-A., Weigand, M., Kläui, M., Bhatia, C. S., Yang, H.

{Scientific Reports}, 5, Nature Publishing Group, London, UK, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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XMCD studies of thin Co films on BaTiO3

Welke, M., Gräfe, J., Govind, R. K., Babu, V. H., Trautmann, M., Schindler, K., Denecke, R.

{Journal of Physics: Condensed Matter}, 27(32), IOP Publishing, Bristol, UK, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Combined FORC and x-ray microscopy study of magnetisation reversal in antidot lattices

Gräfe, J., Haering, F., Stahl, C., Weigand, M., Skripnik, M., Nowak, U., Ziemann, P., Wiedwald, U., Schütz, G., Goering, E.

In IEEE International Magnetics Conference (INTERMAG 2015), IEEE, Beijing, China, 2015 (inproceedings)

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DOI Project Page Project Page [BibTex]

DOI Project Page Project Page [BibTex]


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Low temperature X-ray imaging of magnetic flux patterns in high temperature superconductors

Stahl, C., Ruoß, S., Weigand, M., Bechtel, M., Schütz, G., Albrecht, J.

{Journal of Applied Physics}, 117(17), AIP Publishing, New York, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Local control of domain wall dynamics in ferromagnetic rings

Richter, K., Mawass, M., Krone, A., Krüger, B., Weigand, M., Stoll, H., Schütz, G., Kläui, M.

In IEEE International Magnetics Conference (INTERMAG 2015), IEEE, Beijing, China, 2015 (inproceedings)

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DOI [BibTex]

DOI [BibTex]


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Isosteric heat of hydrogen adsorption on MOFs: comparison between adsorption calorimetry, sorption isosteric metod, and analytical models

Kloutse, A. F., Zacharia, R., Cossement, D., Chahine, R., Balderas-Xicohténcatl, R., Oh, H., Streppel, B., Schlichtenmayer, M., Hirscher, M.

{Applied Physics A}, 121(4):1417-1424, Springer-Verlag Heidelberg, Heidelberg, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Formation of a quasi-solid structure by intercalated noble gas atoms in pores of CuI-MFU-4l metal-organic framework

Magdysyuk, O. V., Denysenko, D., Weinrauch, I., Volkmer, D., Hirscher, M., Dinnebier, R. E.

{Chemical Communications}, 51(4):714-717, Royal Society of Chemistry, Cambridge, UK, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Burst-mode manipulation of magnonic vortex crystals

Hänze, M., Adolff, C. F., Weigand, M., Meier, G.

{Physical Review B}, 91(10), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Investigations of unusual hard magnetic MnBi LTP phase, utilizing temperature dependent SQUID-FORC

Muralidhar, Shreyas

Universität Stuttgart, Stuttgart, 2015 (mastersthesis)

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[BibTex]

[BibTex]


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Magnetische Röntgenmikroskopie an Hochtemperatur-Supraleitern

Stahl, C.

Universität Stuttgart, Stuttgart (und Cuvillier Verlag, Göttingen), 2015 (phdthesis)

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[BibTex]

[BibTex]


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Focused ion beam micromachining enables novel optics for X-ray microscopy

Keskinbora, K., Sanli, U., Grévent, C., Hirscher, M., Schütz, G.

{Microscopy and Microanalysis}, 21(Suppl 3):1983-1984, Springer-Verlag New York, New York, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Selectable nanopattern arrays for nanolithographic imprint and etch-mask applications

Jeong, H., Mark, A. G., Lee, T., Son, K., Chen, W., Alarcón-Correa, M., Kim, I., Schütz, G., Fischer, P.

{Advanced Science}, 2(2), Wiley-VCH, Weinheim, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Grain boundaries as a source of ferromagnetism and increased solubility of Ni in nanograined ZnO

Straumal, B. B., Mazilkin, A. A., Protasova, S. G., Stakhanova, S. V., Straumal, P. B., Bulatov, M. F., Schütz, G., Tietze, T., Goering, E., Baretzky, B.

{Reviews on Advanced Materials Science}, 41, pages: 61-71, 2015 (article)

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[BibTex]

[BibTex]


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Gyrational modes of benzenelike magnetic vortex molecules

Adolff, C. F., Hänze, M., Pues, M., Weigand, M., Meier, G.

{Physical Review B}, 92(2), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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"Job-Sharing" storage of hydrogen in Ru/Li2O nanocomposites

Fu, L., Tang, K., Oh, H., Kandavel, M., Bräuniger, T., Vinod Chandran, C., Menzel, A., Hirscher, M., Samuelis, D., Maier, J.

{Nano Letters}, 15(6):4170-4175, American Chemical Society, Washington, DC, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Overview of the multilayer-Fresnel zone plate and the kinoform lens development at MPI for Intelligent Systems

Sanli, U., Keskinbora, K., Grévent, C., Schütz, G.

{Proceedings of SPIE}, 9510, SPIE, Bellingham, Washington, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Transition matrix elements for electron-phonon scattering: Phenomenological theory and ab initio electron theory

Illg, C., Haag, M., Müller, B. Y., Czycholl, G., Fähnle, M.

{Physical Review B}, 92(19), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Phase evolution in single-crystalline LiFePO4 followed by in situ scanning X-ray microscopy of a micrometre-sized battery

Ohmer, N., Fenk, B., Samuelis, D., Chen, C., Maier, J., Weigand, M., Goering, E., Schütz, G.

{Nature Communications}, 6, Nature Publishing Group, London, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Nitrogen-rich covalent triazine frameworks as high-performance platforms for selective carbon capture and storage

Hug, S., Stegbauer, L., Oh, H., Hirscher, M., Lotsch, B. V.

{Chemistry of Materials}, 27(23):8001-8010, American Chemical Society, Washington, D.C., 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Voltage-induced magnetic manipulation of a microstructured iron gold multilayer system

Sittig, Robert

Universität Stuttgart, Stuttgart, 2015 (mastersthesis)

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[BibTex]

[BibTex]


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Unique high-temperature performance of highly consensed MnBi permanent magnets

Chen, Y., Gregori, G., Leineweber, A., Qu, F., Chen, C., Tietze, T., Kronmüller, H., Schütz, G., Goering, E.

{Scripta Materialia}, 107, pages: 131-135, Pergamon, Tarrytown, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Multilayer Fresnel zone plates for X-ray microscopy

Sanli, U. T., Keskinbora, K., Grévent, C., Szeghalmi, A., Knez, M., Schütz, G.

{Microscopy and Microanalysis}, 21(Suppl 3):1987-1988, Springer-Verlag New York, New York, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Interfacial dominated ferromagnetism in nanograined ZnO: a \muSR and DFT study

Tietze, T., Audehm, P., Chen, Y., Schütz, G., Straumal, B. B., Protasova, S. G., Mazilkin, A. A., Straumal, P. B., Prokscha, T., Luetkens, H., Salman, Z., Suter, A., Baretzky, B., Fink, K., Wenzel, W., Danilov, D., Goering, E.

{Scientific Reports}, 5, pages: 8871-8876, Nature Publishing Group, London, UK, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Preparation of a ferromagnetic barrier in YBa2Cu3O7-delta thinner than the coherence length

Soltan, S., Albrecht, J., Goering, E., Schütz, G., Mustafa, L., Keimer, B., Habermeier, H.

{Journal of Applied Physics}, 118(22), AIP Publishing, New York, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Microanalytical methods for in-situ high-resolution analysis of rock varnish at the micrometer to nanometer scale

Macholdt, D. S., Jochum, K. P., Pöhlker, C., Stoll, B., Weis, U., Weber, B., Müller, M., Kapl, M., Buhre, S., Kilcoyne, A. L. D., Weigand, M., Scholz, D., Al-Amri, A. M., Andreae, M. O.

{Chemical Geology}, 411, pages: 57-68, Elsevier, Amsterdam, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Chemical composition, microstructure, and hygroscopic properties of aerosol particles at the Zotino Tall Tower Observatory (ZOTTO), Siberia, during a summer campaign

Mikhailov, E. F., Mironov, G. N., Pöhlker, C., Chi, X., Krüger, M., Shiraiwa, M., Förster, J., Pöschl, U., Vlasenko, S. S., Ryshkevich, T. I., Weigand, M., Kilcoyne, A. L. D., Andreae, M.

{Atmospheric Chemistry and Physics}, 15(15):8847-8869, European Geosciences Union, Katlenburg-Lindau, Germany, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Orbital reflectometry of PrNiO3/PrAlO3 superlattices

Wu, M., Benckiser, E., Audehm, P., Goering, E., Wochner, P., Christiani, G., Logvenov, G., Habermeier, H., Keimer, B.

{Physical Review B}, 91(19), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Dynamic domain wall chirality rectification by rotating magnetic fields

Bisig, A., Mawass, M., Stärk, M., Moutafis, C., Rhensius, J., Heidler, J., Gliga, S., Weigand, M., Tyliszczak, T., Van Waeyenberge, B., Stoll, H., Schütz, G., Kläui, M.

{Applied Physics Letters}, 106(12), American Institute of Physics, Melville, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Ultrafast demagnetization after laser pulse irradiation in Ni: Ab-initio electron-phonon scattering and phase space calculations

Illg, C., Haag, M., Fähnle, M.

In Ultrafast Magnetism I. Proceedings of the International Conference UMC 2013, 159, pages: 131-133, Springer Proceedings in Physics, Springer, Strasbourg, 2015 (inproceedings)

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DOI [BibTex]

DOI [BibTex]


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Imaging spin dynamics on the nanoscale using X-ray microscopy

Stoll, H., Noske, M., Weigand, M., Richter, K., Krüger, B., Reeve, R. M., Hänze, M., Adolff, C. F., Stein, F., Meier, G., Kläui, M., Schütz, G.

{Frontiers in Physics}, 3, Frontiers Media, Lausanne, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Magnetic moments induce strong phonon renormalization in FeSi

Krannich, S., Sidis, Y., Lamago, D., Heid, R., Mignot, J., von Löhneysen, H., Ivanov, A., Steffens, P., Keller, T., Wang, L., Goering, E., Weber, F.

{Nature Communications}, 6, Nature Publishing Group, London, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Transfer of angular momentum from the spin system to the lattice during ultrafast magnetization

Tsatsoulis, T.

Universität Stuttgart, Stuttgart, 2015 (mastersthesis)

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[BibTex]

[BibTex]


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Electrical determination of vortex state in submicron magnetic elements

Gangwar, A., Bauer, H. G., Chauleau, J., Noske, M., Weigand, M., Stoll, H., Schütz, G., Back, C. H.

{Physical Review B}, 91(9), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Mechanisms for the symmetric and antisymmetric switching of a magnetic vortex core: Differences and common aspects

Noske, M., Stoll, H., Fähnle, M., Hertel, R., Schütz, G.

{Physical Review B}, 91(1), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Automotive domain wall propagation in ferromagnetic rings

Richter, K., Mawass, M., Krone, A., Krüger, B., Weigand, M., Schütz, G., Stoll, H., Kläui, M.

In IEEE International Magnetics Conference (INTERMAG 2015), IEEE, Beijing, China, 2015 (inproceedings)

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DOI [BibTex]

DOI [BibTex]


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High resolution, high efficiency mulitlayer Fresnel zone plates for soft and hard X-rays

Sanli, U., Keskinbora, K., Gregorczyk, K., Leister, J., Teeny, N., Grévent, C., Knez, M., Schütz, G.

{Proceedings of SPIE}, 9592, SPIE, Bellingham, Washington, 2015 (article)

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DOI [BibTex]

DOI [BibTex]


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Macroscopic drift current in the inverse Faraday effect

Hertel, R., Fähnle, M.

{Physical Review B}, 91(2), American Physical Society, Woodbury, NY, 2015 (article)

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DOI [BibTex]

DOI [BibTex]