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2016


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Structure and dynamics of binary liquid mixtures near their continuous demixing transitions

Roy, S., Höfling, F., Dietrich, S.

The Journal of Chemical Physics, 145(4), American Institute of Physics, Woodbury, N.Y., October 2016 (article)

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DOI [BibTex]

2016


DOI [BibTex]


{Coercivity scaling in antidot lattices in Fe, Ni, and NiFe thin films}
Coercivity scaling in antidot lattices in Fe, Ni, and NiFe thin films

Gräfe, J., Schütz, G., Goering, E. J.

{Journal of Magnetism and Magnetic Materials}, 419, pages: 517-520, North-Holland, Amsterdam, 2016 (article)

Abstract
Antidot lattices can be used to artificially engineer magnetic properties in thin films, however, a conclusive model that describes the coercivity enhancement in this class of magnetic nano-structures has so far not been found. We prepared Fe, Ni, and NiFe thin films and patterned each with 21 square antidot lattices with different geometric parameters and measured their hysteretic behavior. On the basis of this extensive dataset we are able to provide a model that can describe both the coercivity scaling over a wide range of geometric lattice parameters and the influence of different materials.

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DOI Project Page [BibTex]

DOI Project Page [BibTex]


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Self-diffusiophoresis of chemically active colloids

Popescu, M. N., Uspal, W. E., Dietrich, S.

The European Physical Journal Special Topics, 225(11-12):2189-2206, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Perpetual superhydrophobicity

Giacomello, A., Schimmele, L., Dietrich, S., Tasinkevych, M.

Soft Matter, 12, pages: 8927-8934, Royal Society of Chemistry, Cambridge, UK, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Molecular dynamics simulation of a binary mixture near the lower critical point

Pousaneh, F., Edholm, O., Maciolek, A.

The Journal of Chemical Physics, 145(1), American Institute of Physics, Woodbury, N.Y., 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Effective Interaction between Active Colloids and Fluid Interfaces Induced by Marangoni Flows

Dom\’\inguez, A., Malgaretti, P., Popescu, M. N., Dietrich, S.

Physical Review Letters, 116, American Physical Society, Woodbury, N.Y., 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Dynamics of Novel Photoactive AgCl Microstars and Their Environmental Applications

Simmchen, J., Baeza, A., Miguel-Lopez, A., Stanton, M. M., Vallet-Regi, M., Ruiz-Molina, D., Sánchez, S.

ChemNanoMat, 3(1):65-71, Wiley, Weinheim, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Wetting hysteresis induced by nanodefects

Giacomello, A., Schimmele, L., Dietrich, S.

Proceedings of the National Academy of Sciences of the United States of America, 113(3):E262-E271, National Academy of Sciences, Washington, D.C., 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Three-phase contact line and line tension of electrolyte solutions in contact with charged substrates

Ibagon, I., Bier, M., Dietrich, S.

Journal of Physics: Condensed Matter, 28(24), IOP Publishing, Bristol, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Smart biosensors for multiplexed and fully integrated point-of-care diagnostics

Romeo, A., Leung, T. S., Sanchez, S.

Lab on a Chip, 16(11):1957-1961, Royal Society of Chemistry, Cambridge, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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The sequential activation of the mitotic microtubule assembly pathways favors bipolar spindle formation

Cavazza, T., Malgaretti, P., Vernos, I.

Molecular Biology of the Cell, 27(19):2935-2945, American Society for Cell Biology, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Entropically induced asymmetric passage times of charged tracers across corrugated channels

Malgaretti, P., Pagonabarraga, I., Rubi, J. M.

The Journal of Chemical Physics, 144(3), American Institute of Physics, Woodbury, N.Y., 2016 (article)

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DOI [BibTex]

DOI [BibTex]


Probabilistic Duality for Parallel Gibbs Sampling without Graph Coloring
Probabilistic Duality for Parallel Gibbs Sampling without Graph Coloring

Mescheder, L., Nowozin, S., Geiger, A.

Arxiv, 2016 (article)

Abstract
We present a new notion of probabilistic duality for random variables involving mixture distributions. Using this notion, we show how to implement a highly-parallelizable Gibbs sampler for weakly coupled discrete pairwise graphical models with strictly positive factors that requires almost no preprocessing and is easy to implement. Moreover, we show how our method can be combined with blocking to improve mixing. Even though our method leads to inferior mixing times compared to a sequential Gibbs sampler, we argue that our method is still very useful for large dynamic networks, where factors are added and removed on a continuous basis, as it is hard to maintain a graph coloring in this setup. Similarly, our method is useful for parallelizing Gibbs sampling in graphical models that do not allow for graph colorings with a small number of colors such as densely connected graphs.

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pdf [BibTex]


γ‐Conicein und Coniin aus Geflecktem Schierling
γ‐Conicein und Coniin aus Geflecktem Schierling

Puidokait, M., Graefe, J., Sehl, A., Steinke, K., Siehl, H., Zeller, K., Sicker, D., Berger, S.

Chemie in unserer Zeit, 50(6):382-391, 2016 (article)

Abstract
Sokrates ist das bekannteste Opfer eines 399 v.d.Z. in Athen mit dem Schierlingsbecher vollstreckten Todesurteils. Tödlich giftig wirkten darin Alkaloide wie γ‐Conicein und Coniin, die nach Mäuseurin riechen. Schaudern macht, dass dieses Gift sein Opfer allmählich bei vollem Bewusstsein lähmt und dass es kein Gegengift gibt. Auch für Tiere auf der Weide ist Gefleckter Schierling stark giftig. Daher verdrängt die Landwirtschaft den Schierling. Coniin war das erste synthetisierte Alkaloid (Ladenburg, 1886). Schierlingsgifte werden heute nicht medizinisch angewendet. Wir beschreiben die Isolierung von γ‐Conicein und Coniin aus angebautem und wildem Gefleckten Schierling und analysieren ihre Struktur spektroskopisch. Dieser Artikel gehört zur Reihe über die Isolierung und Spektroskopie von Naturstoffen und ergänzt die Kapitel des Buchs “Classics in Spectroscopy” von S. Berger und D. Sicker (Wiley‐VCH 2009). Er beruht auf studentischen Arbeiten ebenso wie auf unserem präparativen Engagement als sie betreuende Wissenschaftler.

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DOI [BibTex]

DOI [BibTex]


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Topographical pathways guide chemical microswimmers

Simmchen, J., Katuri, J., Uspal, W., Popescu, M. N., Tasinkevych, M., Sanchez, S.

Nature Communications, 7, Nature Publishing Group, London, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Fluctuational electrodynamics for nonlinear media

Soo, H., Krüger, M.

EPL, 115(4), EDP Science, Les-Ulis, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Poisson-Boltzmann study of the effective electrostatic interaction between colloids at an electrolyte interface

Majee, A., Bier, M., Dietrich, S.

The Journal of Chemical Physics, 145(6), American Institute of Physics, Woodbury, N.Y., 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Bubble-Free Propulsion of Ultrasmall Tubular Nanojets Powered by Biocatalytic Reactions

Ma, X., Hortelao, A. C., Miquel-Lopez, A., Sanchez, S.

Journal of the American Chemical Society, 138(42):13782-13785, American Chemical Society, Washington, DC, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Wetting and orientation of catalytic Janus colloids at the surface of water

Wang, X., In, M., Blanc, C., Malgaretti, P., Nobilia, M., Stocco, A.

Faraday Discussions, 191, pages: 305-324, Royal Society of Chemistry, London, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Collective dynamics of chemically active particles trapped at a fluid interface

Dom\’\inguez, A., Malgaretti, P., Popescu, M. N., Dietrich, S.

Soft Matter, 12(40):8398-8406, Royal Society of Chemistry, Cambridge, UK, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Guiding Catalytically Active Particles with Chemically Patterned Surfaces

Uspal, W. E., Popescu, M. N., Dietrich, S., Tasinkevych, M.

Physical Review Letters, 117(4), American Physical Society, Woodbury, N.Y., 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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A dynamic DFT approach to generalized diffusion equations in a system with long-ranged and hydrodynamic interactions

Bleibel, J., Dominguez, A., Oettel, M.

Journal of Physics: Condensed Matter, 28(24), IOP Publishing, Bristol, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Rectification and Non-Gaussian Diffusion in Heterogeneous Media

Malgaretti, P., Pagonabarraga, I., Rubi, J. M.

Entropy, 18(11), Molecular Diversity Preservation International, Basel, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Lateral critical Casimir force in two\textendashdimensional inhomogeneous Ising strip. Exact results

Nowakowski, P., Napiorkowski, M.

The Journal of Chemical Physics, 144(21), 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Tailoring three-dimensional architectures by rolled-up nanotechnology for mimicking microvasculatures

Arayanarakool, R., Meyer, A. K., Helbig, L., Sanchez, S., Schmidt, O. G.

Lab on a Chip, 15(14):2981-2989, Royal Society of Chemistry, Cambridge, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Flexible sensors for biomedical technology

Vilela, D., Romeo, A., Sanchez, S.

Lab on a Chip, 16(3):402-408, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Mechanical stability of bipolar spindle assembly

Malgaretti, P., Muhuri, S.

EPL, 115(2), EDP Science, Les-Ulis, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Reversed Janus micro/nanomotors with internal chemical engine

Ma, X., Jang, S., Popescu, M. N., Uspal, W. E., Miguel-López, A., Hahn, K., Kim, D., Sanchez, S.

ACS Nano, 10(9):8751-8759, American Chemical Society, Washington, DC, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Driven colloidal fluids: construction of dynamical density functional theories from exactly solvable limits

Scacchi, A., Krüger, M., Brader, J. M.

Journal of Physics: Condensed Matter, 28(24), IOP Publishing, Bristol, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Flight of a heavy particle nonlinearly coupled to a quantum bath

Maghrebi, M. F., Krüger, M., Kardar, M.

Physical Review B, 93(1), American Physical Society, Woodbury, NY, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Critical Casimir forces between defects in the 2D Ising model

Nowakowski, P., Maciolek, A., Dietrich, S.

Journal of Physics A: Mathematical and Theoretical, 49(48), IOP Pub., Bristol, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Miniaturized soft bio-hybrid robotics: a step forward into healthcare applications

Patino, T., Mestre, R., Sanchez, S.

Lab on a Chip, 16(19):3626-3630, Royal Society of Chemistry, Cambridge, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Characterizing anomalous diffusion in crowded polymer solutions and gels over five decades in time with variable-lengthscale fluorescence correlation spectroscopy

Banks, Daniel S, Tressler, Charmaine, Peters, Robert D, Höfling, Felix, Fradin, Cécile

Soft Matter, 12(18):4190-4203, Royal Society of Chemistry, Cambridge, UK, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Slip Length Enhancement in Nanofluidic Flow using Nanotextured Superhydrophobic Surfaces

Heverhagen, Jonas, Tasinkevych, M., Rahman, A., Black, C.T., Checco, A.

Advanced Materials Interfaces, 3(17), Wiley-VCH, Weinheim, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


{Geometric control of the magnetization reversal in antidot lattices with perpendicular magnetic anisotropy}
Geometric control of the magnetization reversal in antidot lattices with perpendicular magnetic anisotropy

Gräfe, J., Weigand, M., Träger, N., Schütz, G., Goering, E. J., Skripnik, M., Nowak, U., Haering, F., Ziemann, P., Wiedwald, U.

{Physical Review B}, 93(10), American Physical Society, Woodbury, NY, 2016 (article)

Abstract
While the magnetic properties of nanoscaled antidot lattices in in-plane magnetized materials have widely been investigated, much less is known about the microscopic effect of hexagonal antidot lattice patterning on materials with perpendicular magnetic anisotropy. By using a combination of first-order reversal curve measurements, magnetic x-ray microscopy, and micromagnetic simulations we elucidate the microscopic origins of the switching field distributions that arise from the introduction of antidot lattices into out-of-plane magnetized GdFe thin films. Depending on the geometric parameters of the antidot lattice we find two regimes with different magnetization reversal processes. For small antidots, the reversal process is dominated by the exchange interaction and domain wall pinning at the antidots drives up the coercivity of the system. On the other hand, for large antidots the dipolar interaction is dominating which leads to fragmentation of the system into very small domains that can be envisaged as a basis for a bit patterned media.

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DOI Project Page Project Page [BibTex]

DOI Project Page Project Page [BibTex]


{Magnetic switching of nanoscale antidot lattices}
Magnetic switching of nanoscale antidot lattices

Wiedwald, U., Gräfe, J., Lebecki, K. M., Skripnik, M., Haering, F., Schütz, G., Ziemann, P., Goering, E., Nowak, U.

{Beilstein Journal of Nanotechnology}, 7, pages: 733-750, Beilstein-Institut, Frankfurt am Main, 2016 (article)

Abstract
We investigate the rich magnetic switching properties of nanoscale antidot lattices in the 200 nm regime. In-plane magnetized Fe, Co, and Permalloy (Py) as well as out-of-plane magnetized GdFe antidot films are prepared by a modified nanosphere lithography allowing for non-close packed voids in a magnetic film. We present a magnetometry protocol based on magneto-optical Kerr microscopy elucidating the switching modes using first-order reversal curves. The combination of various magnetometry and magnetic microscopy techniques as well as micromagnetic simulations delivers a thorough understanding of the switching modes. While part of the investigations has been published before, we summarize these results and add significant new insights in the magnetism of exchange-coupled antidot lattices.

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DOI Project Page [BibTex]

DOI Project Page [BibTex]


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Active colloids at fluid interfaces

Malgaretti, P., Popescu, M. N., Dietrich, S.

Soft Matter, 12(17):4007-4023, Royal Society of Chemistry, Cambridge, UK, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Critical adsorption and critical Casimir forces in the canonical ensemble

Gross, M., Vasilyev, O., Gambassi, A., Dietrich, S.

Physical Review E, 94(2), American Physical Society, Melville, NY, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Critical Casimir interactions between Janus particles

Labbe-Laurent, M., Dietrich, S.

Soft Matter, 12(31):6621-6648, Royal Society of Chemistry, Cambridge, UK, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Motion Control of Urea-Powerde Biocompatible Hollow Microcapsule

Ma, X., Wang, X., Hahn, K., Sanchez, S.

ACS Nano, 10(3):3597-3605, American Chemical Society, Washington, DC, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Enzyme Catalysis To Power Micro/Nanomachines

Ma, X., Hortelao, A. C., Patino, T., Sanchez, S.

ACS Nano, 10(10):9111-9122, American Chemical Society, Washington, DC, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Microfluidic fuel cells for energy generation

Safdar, M., Jänis, J., Sanchez, S.

Lab on a Chip, 16(15):2754-2758, Royal Society of Chemistry, Cambridge, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Reusable and Long-Lasting Active Microcleaners for Heterogeneous Water Remediation

Parmar, J., Vilela, D., Pellicer, E., Esque-de-los Ojos, D., Sort, J., Sanchez, S.

Advanced Functional Materials, 26(23):4152-4161, Wiley-VCH Verlag GmbH, Weinheim, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Self-Assembly of Micromachining Systems Powered by Janus Micromotors

Maggi, C., Simmchen, J., Saglimbeni, F., Katuri, J., Dipalo, M., De Angelis, F., Sanchez, S., Di Leonardo, R.

Small, 12(4):446-451, Wiley, Weinheim, Germany, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Graphene-Based Microrobots for Toxic Heavy Metal Removal and Recovery from Water

Vilela, D., Parmar, J., Zeng, Y., Zhao, Y., Sanchez, S.

Nano Letters, 16(4):2860-2866, American Chemical Society, Washington, DC, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


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Colloidal Particles in Thin Nematic Wetting Films

Jeridi, H., Tasinkevych, M., Othman, T., Blanc, C.

Langmuir, 32(35):9097-9107, American Chemical Society, Columbus, OH, 2016 (article)

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DOI [BibTex]

DOI [BibTex]


Map-Based Probabilistic Visual Self-Localization
Map-Based Probabilistic Visual Self-Localization

Brubaker, M. A., Geiger, A., Urtasun, R.

IEEE Trans. on Pattern Analysis and Machine Intelligence (PAMI), 2016 (article)

Abstract
Accurate and efficient self-localization is a critical problem for autonomous systems. This paper describes an affordable solution to vehicle self-localization which uses odometry computed from two video cameras and road maps as the sole inputs. The core of the method is a probabilistic model for which an efficient approximate inference algorithm is derived. The inference algorithm is able to utilize distributed computation in order to meet the real-time requirements of autonomous systems in some instances. Because of the probabilistic nature of the model the method is capable of coping with various sources of uncertainty including noise in the visual odometry and inherent ambiguities in the map (e.g., in a Manhattan world). By exploiting freely available, community developed maps and visual odometry measurements, the proposed method is able to localize a vehicle to 4m on average after 52 seconds of driving on maps which contain more than 2,150km of drivable roads.

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pdf Project Page [BibTex]

pdf Project Page [BibTex]


{Combined first-order reversal curve and x-ray microscopy investigation of magnetization reversal mechanisms in hexagonal antidot lattices}
Combined first-order reversal curve and x-ray microscopy investigation of magnetization reversal mechanisms in hexagonal antidot lattices

Gräfe, J., Weigand, M., Stahl, C., Träger, N., Kopp, M., Schütz, G., Goering, E. J., Haering, F., Ziemann, P., Wiedwald, U.

{Physical Review B}, 93(1), American Physical Society, Woodbury, NY, 2016 (article)

Abstract
The magnetization reversal in nanoscaled antidot lattices is widely investigated to understand the tunability of the magnetic anisotropy and the coercive field through nanostructuring of thin films. By investigating highly ordered focused ion beam milled antidot lattices with a combination of first-order reversal curves and magnetic x-ray microscopy, we fully elucidate the magnetization reversal along the distinct orientations of a hexagonal antidot lattice. This combination proves especially powerful as all partial steps of this complex magnetization reversal can be identified and subsequently imaged. Through this approach we discovered several additional steps that were neglected in previous studies. Furthermore, by imaging the microscopic magnetization state during each reversal step, we were able to link the coercive and interaction fields determined by the first-order reversal curve method to true microscopic magnetization configurations and determine their origin.

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DOI Project Page Project Page [BibTex]

DOI Project Page Project Page [BibTex]


{Switching probabilities of magnetic vortex core reversal studied by table top magneto optic Kerr microscopy}
Switching probabilities of magnetic vortex core reversal studied by table top magneto optic Kerr microscopy

Dieterle, G., Gangwar, A., Gräfe, J., Noske, M., Förster, J., Woltersdorf, G., Stoll, H., Back, C. H., Schütz, G.

{Applied Physics Letters}, 108(2), American Institute of Physics, Melville, NY, 2016 (article)

Abstract
We have studied vortex core reversal in a single submicron Permalloy disk by polar Kerr microscopy. A sophisticated lock-in-technique based on repetitive switching of the magnetic vortex core and a continuous calibration allows for a reliable determination of the switching probability. This highly sensitive method facilitates the detection of a change in the magnetic moment of the tiny magnetic vortex core which is about 1.5 × 10−17 A m2. We have investigated vortex core switching caused by excitation of the vortex core gyromode with varying frequencies and amplitudes. The frequency range in which switching occurs was found to broaden with increasing excitation amplitude, whereby the highest frequency in this range shifts stronger to higher frequencies than the lowest frequency to lower frequencies. The experimental results are in good agreement with micromagnetic simulations.

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DOI [BibTex]

DOI [BibTex]


{Pinned orbital moments - A new contribution to magnetic anisotropy}
Pinned orbital moments - A new contribution to magnetic anisotropy

Audehm, P., Schmidt, M., Brück, S., Tietze, T., Gräfe, J., Macke, S., Schütz, G., Goering, E.

{Scientific Reports}, 6, Nature Publishing Group, London, UK, 2016 (article)

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DOI [BibTex]

DOI [BibTex]