Header logo is


2020


Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles
Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles

Singh, D., Domínguez, A., Choudhury, U., Kottapalli, S., Popescu, M., Dietrich, S., Fischer, P.

Nature Communications, 11(2210), May 2020 (article)

Abstract
Symmetry breaking and the emergence of self-organized patterns is the hallmark of com- plexity. Here, we demonstrate that a sessile drop, containing titania powder particles with negligible self-propulsion, exhibits a transition to collective motion leading to self-organized flow patterns. This phenomenology emerges through a novel mechanism involving the interplay between the chemical activity of the photocatalytic particles, which induces Mar- angoni stresses at the liquid–liquid interface, and the geometrical confinement provided by the drop. The response of the interface to the chemical activity of the particles is the source of a significantly amplified hydrodynamic flow within the drop, which moves the particles. Furthermore, in ensembles of such active drops long-ranged ordering of the flow patterns within the drops is observed. We show that the ordering is dictated by a chemical com- munication between drops, i.e., an alignment of the flow patterns is induced by the gradients of the chemicals emanating from the active particles, rather than by hydrodynamic interactions.

pf icm

link (url) DOI [BibTex]


no image
Wetting transitions on soft substrates

Napiorkowski, M., Schimmele, L., Dietrich, S.

{EPL}, 129(1), EDP Science, Les-Ulis, 2020 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Blessing and Curse: How a Supercapacitor Large Capacitance Causes its Slow Charging

Lian, C., Janssen, M., Liu, H., van Roij, R.

Physical Review Letters, 124(7), American Physical Society, Woodbury, N.Y., 2020 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Fractal-seaweeds type functionalization of graphene

Amsharov, K., Sharapa, D. I., Vasilyev, O. A., Martin, O., Hauke, F., Görling, A., Soni, H., Hirsch, A.

Carbon, 158, pages: 435-448, Elsevier, Amsterdam, 2020 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Energy storage in steady states under cyclic local energy input

Zhang, Y., Holyst, R., Maciolek, A.

Physical Review E, 101(1), American Physical Society, Melville, NY, 2020 (article)

icm

DOI [BibTex]

DOI [BibTex]

2019


no image
Response of active Brownian particles to shear flow

Asheichyk, K., Solon, A., Rohwer, C. M., Krüger, M.

The Journal of Chemical Physics, 150(14), American Institute of Physics, Woodbury, N.Y., 2019 (article)

icm

DOI [BibTex]

2019


DOI [BibTex]


no image
Vortex Mass in the Three-Dimensional O(2) Scalar Theory

Delfino, G., Selke, W., Squarcini, A.

Physical Review Letters, 122(5), American Physical Society, Woodbury, N.Y., 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Ferromagnetic colloids in liquid crystal solvents

Zarubin, G.

Universität Stuttgart, Stuttgart, 2019 (phdthesis)

icm

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
Fluctuating interface with a pinning potential

Pranjić, Daniel

Universität Stuttgart, Stuttgart, 2019 (mastersthesis)

icm

[BibTex]

[BibTex]


no image
Dynamics near planar walls for various model self-phoretic particles

Bayati, P., Popescu, M. N., Uspal, W. E., Dietrich, S., Najafi, A.

Soft Matter, 15(28):5644-5672, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Glucose Oxidase Micropumps: Multi-Faceted Effects of Chemical Activity on Tracer Particles Near the Solid-Liquid Interface

Munteanu, R. E., Popescu, M. N., Gáspár, S.

Condensed Matter, 4(3), MDPI, Basel, 2019 (article)

icm

DOI [BibTex]


no image
Criticality senses topology

Vasilyev, O. A., Maciolek, A., Dietrich, S.

EPL, 128(2), EDP Science, Les-Ulis, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Drag Force for Asymmetrically Grafted Colloids in Polymer Solutions

Werner, M., Malgaretti, P., Maciolek, A.

Frontiers in Physics, 7, Frontiers Media, Lausanne, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Feeling Your Neighbors across the Walls: How Interpore Ionic Interactions Affect Capacitive Energy Storage

Kondrat, S., Vasilyev, O., Kornyshev, A. A.

The Journal of Physical Chemistry Letters, 10(16):4523-4527, American Chemical Society, Washington, DC, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Active Janus colloids at chemically structured surfaces

Uspal, W. E., Popescu, M. N., Dietrich, S., Tasinkevych, M.

The Journal of Chemical Physics, 150(20), American Institute of Physics, Woodbury, N.Y., 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Illumination-induced motion of a Janus nanoparticle in binary solvents

Araki, T., Maciolek, A.

Soft Matter, 15(26):5243-5254, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Transient response of an electrolyte to a thermal quench

Janssen, M., Bier, M.

Physical Review E, 99(4), American Physical Society, Melville, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Aging phenomena during phase separation in fluids: decay of autocorrelation for vapor\textendashliquid transitions

Roy, Sutapa, Bera, Arabinda, Majumder, Suman, Das, Subir K.

Soft Matter, 15(23):4743-4750, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Controlling pattern formation in the confined Schnakenberg model

Beyer, David Bernhard

Universität Stuttgart, Stuttgart, 2019 (mastersthesis)

icm

[BibTex]

[BibTex]


no image
Flux and storage of energy in nonequilibrium stationary states

Holyst, R., Maciolek, A., Zhang, Y., Litniewski, M., Knycha\la, P., Kasprzak, M., Banaszak, M.

Physical Review E, 99(4), American Physical Society, Melville, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Correlations and forces in sheared fluids with or without quenching

Rohwer, C. M., Maciolek, A., Dietrich, S., Krüger, M.

New Journal of Physics, 21, IOP Publishing, Bristol, 2019 (article)

icm

DOI [BibTex]


no image
Ensemble dependence of critical Casimir forces in films with Dirichlet boundary conditions

Rohwer, C. M., Squarcini, A., Vasilyev, O., Dietrich, S., Gross, M.

Physical Review E, 99(6), American Physical Society, Melville, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Controlling the dynamics of colloidal particles by critical Casimir forces

Magazzù, A., Callegari, A., Staforelli, J. P., Gambassi, A., Dietrich, S., Volpe, G.

Soft Matter, 15(10):2152-2162, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Charge regulation radically modifies electrostatics in membrane stacks

Majee, A., Bier, M., Blossey, R., Podgornik, R.

Physical Review E, 100(5), American Physical Society, Melville, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Comment on "Which interactions dominate in active colloids?" [J. Chem. Phys. 150, 061102 (2019)]

Popescu, M. N., Dominguez, A., Uspal, W. E., Tasinkevych, M., Dietrich, S.

The Journal of Chemical Physics, 151(6), American Institute of Physics, Woodbury, N.Y., 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Current-mediated synchronization of a pair of beating non-identical flagella

Dotsenko, V., Maciolek, A., Oshanin, G., Vasilyev, O., Dietrich, S.

New Journal of Physics, 21, IOP Publishing, Bristol, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Driving an electrolyte through a corrugated nanopore

Malgaretti, P., Janssen, M., Pagonabarraga, I., Rubi, J. M.

The Journal of Chemical Physics, 151(8), American Institute of Physics, Woodbury, N.Y., 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Interfaces in fluids of ionic liquid crystals

Bartsch, H.

Universität Stuttgart, Stuttgart, 2019 (phdthesis)

icm

link (url) DOI [BibTex]

link (url) DOI [BibTex]


no image
Spectral Content of a Single Non-Brownian Trajectory

Krapf, D., Lukat, N., Marinari, E., Metzler, R., Oshanin, G., Selhuber-Unkel, C., Squarcini, A., Stadler, L., Weiss, M., Xu, X.

Physical Review X, 9(1), American Physical Society, New York, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Curvature affects electrolyte relaxation: Studies of spherical and cylindrical electrodes

Janssen, M.

Physical Review E, 100(4), American Physical Society, Melville, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Dynamics of the critical Casimir force for a conserved order parameter after a critical quench

Gross, M., Rohwer, C. M., Dietrich, S.

Physical Review E, 100(1), American Physical Society, Melville, NY, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Interface structures in ionic liquid crystals

Bartsch, H., Bier, M., Dietrich, S.

Soft Matter, 15(20):4109-4126, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Interfacial premelting of ice in nano composite materials

Li, H., Bier, M., Mars, J., Weiss, H., Dippel, A., Gutowski, O., Honkimäki, V., Mezger, M.

Physical Chemistry Chemical Physics, 21(7):3734-3741, Royal Society of Chemistry, Cambridge, England, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Connections Matter: On the Importance of Pore Percolation for Nanoporous Supercapacitors

Vasilyev, O., Kornyshev, A. A., Kondrat, S.

ACS Applied Energy Materials, 2(8):5386-5390, American Chemical Society, Washington, DC, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Theory of light-activated catalytic Janus particles

Uspal, W. E.

The Journal of Chemical Physics, 150(11), American Institute of Physics, Woodbury, N.Y., 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Recovering superhydrophobicity in nanoscale and macroscale surface textures

Giacomello, A., Schimmele, L., Dietrich, S., Tasinkevych, M.

Soft Matter, 15(37):7462-7471, Royal Society of Chemistry, Cambridge, UK, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Brownian dynamics assessment of enhanced diffusion exhibited by "fluctuating-dumbbell enzymes".

Kondrat, S., Popescu, M. N.

Physical Chemistry Chemical Physics, 21(35):18811-18815, Royal Society of Chemistry, Cambridge, England, 2019 (article)

icm

DOI [BibTex]

DOI [BibTex]

2014


no image
Ultracompact Three-Dimensional Tubular Conductivity Microsensors for Ionic and Biosensing Applications

Martinez-Cisneros, C. S., Sanchez, S., Schmidt, O. G., Xi, W.

Nano Letters, pages: 2219-2224, American Chemical Society, Washington, DC, 2014 (article)

Abstract
We present ultracompact three-dimensional tubular structures integrating Au-based electrodes as impedimetric microsensors for the in-flow determination of mono- and divalent ionic species and HeLa cells. The microsensors show an improved performance of 2 orders of magnitude (limit of detection \textequals 0.1 nM for KCl) compared to conventional planar conductivity detection systems integrated in microfluidic platforms and the capability to detect single HeLa cells in flowing phosphate buffered saline. These highly integrated conductivity tubular sensors thus open new possibilities for lab-in-a-tube devices for bioapplications such as biosensing and bioelectronics.

icm

DOI [BibTex]

2014


DOI [BibTex]


no image
Catalytic nanomotors for environmental monitoring and water remediation

Soler, L., Sanchez, S.

Nanoscale, 6(13):7175-7182, 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Proton-proton collisions at ultra-relativistic energies in quark-gluon string model

Bravina, L., Bleibel, J., Malinina, L., Nilsson, M. S., Zabrodin, E.

EPJ Web of Conferences, 70, EDP Sciences, Les Ulis, 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Hydrodynamic interactions induce anomalous diffusion under partial confinement

Bleibel, J., Dominguez, A., Günther, F., Harting, J., Oettel, M.

Soft Matter, 10(17):2945-2948, Royal Society of Chemistry, Cambridge, UK, 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Clay nanotube encapsulation for functional biocomposites

Lvov, Y., Aerov, Artem A., Aerov, A. A., Fakhrullin, R.

Advances in Colloid and Interface Science, 207, pages: 189-198, 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Wetting phenomena in electrolyte solutions

Ibagon, I.

Universität Stuttgart, Stuttgart, 2014 (phdthesis)

icm

link (url) [BibTex]

link (url) [BibTex]


no image
Control of Self-Propelled Microjets Inside a Microchannel With Time-Varying Flow Rates

Magdanz, V., Sanchez, S., Schmidt, O. G., Khalil, I. S. M., Misra, S.

IEEE Transactions on Robotics and Automation, pages: 49-58, IEEE, New York, NY, 2014 (article)

Abstract
We demonstrate the closed-loop motion control of self-propelled microjets inside a fluidic microchannel. The motion control of the microjets is achieved in hydrogen peroxide solution with time-varying flow rates, under the influence of the controlled magnetic fields and the self-propulsion force. Magnetic dipole mo- ment of the microjets is characterized using the U-turn and the rotating field techniques. The characterized magnetic dipole mo- ment has an average of 1.4 $\times$ 10 \textminus 13 A.m 2 at magnetic field, linear velocity, and boundary frequency of 2 mT, 100 $\mu$ m/s, and 25 rad/s, respectively. We implement a closed-loop control system that is based on the characterized magnetic dipole moment of the mi- crojets. This closed-loop control system positions the microjets by directing the magnetic field lines toward the reference position. Experiments are done using a magnetic system and a fluidic mi- crochannel with a width of 500 $\mu$ m. In the absence of a fluid flow, our control system positions the microjets at an average velocity and within an average region-of-convergence (ROC) of 119 $\mu$ m/s and 390 $\mu$ m, respectively. As a representative case, we observe that our control system positions the microjets at an average velocity and within an average ROC of 90 $\mu$ m/s and 600 $\mu$ m and 120 $\mu$ m/s and 600 $\mu$ m when a flow rate of 2.5 $\mu$ l/min is applied against and along the direction of the microjets, respectively. Furthermore, the average velocity and ROC are determined throughout the flow range (0 to 7.5 $\mu$ l/min) to characterize the motion of the microjets inside the microchannel

icm

DOI [BibTex]

DOI [BibTex]


no image
Electrostatic interaction between colloidal particles trapped at an electrolyte interface

Majee, A., Bier, M., Dietrich, S.

The Journal of Chemical Physics, 140(16), American Institute of Physics, Woodbury, N.Y., 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Capillary attraction induced collapse of colloidal monolayers at fluid interfaces

Bleibel, J., Dominguez, A., Oettel, M., Dietrich, S.

Soft Matter, 10(23):4091-4109, Royal Society of Chemistry, Cambridge, UK, 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Trapping self-propelled micromotors with microfabricated chevron and heart-shaped chips

Restrepo-Pérez, L., Soler, L., Mart\’\inez-Cisneros, C. S., Sanchez, S., Schmidt, O. G.

Lab on a Chip, 14(9):1515-1518, 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]


no image
Order of wetting transitions in electrolyte solutions

Ibagon, I., Bier, M., Dietrich, S.

The Journal of Chemical Physics, 140(17), American Institute of Physics, Woodbury, N.Y., 2014 (article)

icm

DOI [BibTex]

DOI [BibTex]