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2020


Statistical reprogramming of macroscopic self-assembly with dynamic boundaries
Statistical reprogramming of macroscopic self-assembly with dynamic boundaries

Culha, U., Davidson, Z. S., Mastrangeli, M., Sitti, M.

Proceedings of the National Academy of Sciences, 117(21):11306-11313, May 2020 (article)

Abstract
Self-assembly is a ubiquitous process that can generate complex and functional structures via local interactions among a large set of simpler components. The ability to program the self-assembly pathway of component sets elucidates fundamental physics and enables alternative competitive fabrication technologies. Reprogrammability offers further opportunities for tuning structural and material properties but requires reversible selection from multistable self-assembling patterns, which remains a challenge. Here, we show statistical reprogramming of two-dimensional (2D), noncompact self-assembled structures by the dynamic confinement of orbitally shaken and magnetically repulsive millimeter-scale particles. Under a constant shaking regime, we control the rate of radius change of an assembly arena via moving hard boundaries and select among a finite set of self-assembled patterns repeatably and reversibly. By temporarily trapping particles in topologically identified stable states, we also demonstrate 2D reprogrammable stiffness and three-dimensional (3D) magnetic clutching of the self-assembled structures. Our reprogrammable system has prospective implications for the design of granular materials in a multitude of physical scales where out-of-equilibrium self-assembly can be realized with different numbers or types of particles. Our dynamic boundary regulation may also enable robust bottom-up control strategies for novel robotic assembly applications by designing more complex spatiotemporal interactions using mobile robots.

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DOI [BibTex]

2020


DOI [BibTex]


Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles
Interface-mediated spontaneous symmetry breaking and mutual communication between drops containing chemically active particles

Singh, D., Domínguez, A., Choudhury, U., Kottapalli, S., Popescu, M., Dietrich, S., Fischer, P.

Nature Communications, 11(2210), May 2020 (article)

Abstract
Symmetry breaking and the emergence of self-organized patterns is the hallmark of com- plexity. Here, we demonstrate that a sessile drop, containing titania powder particles with negligible self-propulsion, exhibits a transition to collective motion leading to self-organized flow patterns. This phenomenology emerges through a novel mechanism involving the interplay between the chemical activity of the photocatalytic particles, which induces Mar- angoni stresses at the liquid–liquid interface, and the geometrical confinement provided by the drop. The response of the interface to the chemical activity of the particles is the source of a significantly amplified hydrodynamic flow within the drop, which moves the particles. Furthermore, in ensembles of such active drops long-ranged ordering of the flow patterns within the drops is observed. We show that the ordering is dictated by a chemical com- munication between drops, i.e., an alignment of the flow patterns is induced by the gradients of the chemicals emanating from the active particles, rather than by hydrodynamic interactions.

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link (url) DOI [BibTex]


Spectrally selective and highly-sensitive UV photodetection with UV-A, C band specific polarity switching in silver plasmonic nanoparticle enhanced gallium oxide thin-film
Spectrally selective and highly-sensitive UV photodetection with UV-A, C band specific polarity switching in silver plasmonic nanoparticle enhanced gallium oxide thin-film

Arora, K., Singh, D., Fischer, P., Kumar, M.

Adv. Opt. Mat., March 2020 (article)

Abstract
Traditional photodetectors generally show a unipolar photocurrent response when illuminated with light of wavelength equal or shorter than the optical bandgap. Here, we report that a thin film of gallium oxide (GO) decorated with plasmonic nanoparticles, surprisingly, exhibits a change in the polarity of the photocurrent for different UV bands. Silver (Ag) nanoparticles are vacuum-deposited onto β-Ga2O3 and the AgNP@GO thin films show a record responsivity of 250 A/W, which significantly outperforms bare GO planar photodetectors. The photoresponsivity reverses sign from +157 µA/W in the UV-C band under unbiased operation to -353 µA/W in the UV-A band. The current reversal is rationalized by considering the charge dynamics stemming from hot electrons generated when the incident light excites a local surface plasmon resonance (LSPR) in the Ag nanoparticles. The Ag nanoparticles improve the external quantum efficiency and detectivity by nearly one order of magnitude with high values of 1.2×105 and 3.4×1014 Jones, respectively. This plasmon-enhanced solar blind GO detector allows UV regions to be spectrally distinguished, which is useful for the development of sensitive dynamic imaging photodetectors.

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[BibTex]


Acoustofluidic Tweezers for the 3D Manipulation of Microparticles
Acoustofluidic Tweezers for the 3D Manipulation of Microparticles

Guo, X., Ma, Z., Goyal, R., Jeong, M., Pang, W., Fischer, P., Dian, X., Qiu, T.

In 2020 IEEE International Conference on Robotics and Automation (ICRA),, Febuary 2020 (conference)

Abstract
Non-contact manipulation is of great importance in the actuation of micro-robotics. It is challenging to contactless manipulate micro-scale objects over large spatial distance in fluid. Here, we describe a novel approach for the dynamic position control of microparticles in three-dimensional (3D) space, based on high-speed acoustic streaming generated by a micro-fabricated gigahertz transducer. Due to the vertical lifting force and the horizontal centripetal force generated by the streaming, microparticles are able to be stably trapped at a position far away from the transducer surface, and to be manipulated over centimeter distance in all three directions. Only the hydrodynamic force is utilized in the system for particle manipulation, making it a versatile tool regardless the material properties of the trapped particle. The system shows high reliability and manipulation velocity, revealing its potentials for the applications in robotics and automation at small scales.

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[BibTex]

[BibTex]


Investigating photoresponsivity of graphene-silver hybrid nanomaterials in the ultraviolet
Investigating photoresponsivity of graphene-silver hybrid nanomaterials in the ultraviolet

Deshpande, P., Suri, P., Jeong, H., Fischer, P., Ghosh, A., Ghosh, G.

J. Chem. Phys., 152, pages: 044709, January 2020 (article)

Abstract
There have been several reports of plasmonically enhanced graphene photodetectors in the visible and the near infrared regime but rarely in the ultraviolet. In a previous work, we have reported that a graphene-silver hybrid structure shows a high photoresponsivity of 13 A/W at 270 nm. Here, we consider the likely mechanisms that underlie this strong photoresponse. We investigate the role of the plasmonic layer and examine the response using silver and gold nanoparticles of similar dimensions and spatial arrangement. The effect on local doping, strain, and absorption properties of the hybrid is also probed by photocurrent measurements and Raman and UV-visible spectroscopy. We find that the local doping from the silver nanoparticles is stronger than that from gold and correlates with a measured photosensitivity that is larger in devices with a higher contact area between the plasmonic nanomaterials and the graphene layer.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


A High-Fidelity Phantom for the Simulation and Quantitative Evaluation of Transurethral Resection of the Prostate
A High-Fidelity Phantom for the Simulation and Quantitative Evaluation of Transurethral Resection of the Prostate

Choi, E., Adams, F., Gengenbacher, A., Schlager, D., Palagi, S., Müller, P., Wetterauer, U., Miernik, A., Fischer, P., Qiu, T.

Annals of Biomed. Eng., 48, pages: 437-446, January 2020 (article)

Abstract
Transurethral resection of the prostate (TURP) is a minimally invasive endoscopic procedure that requires experience and skill of the surgeon. To permit surgical training under realistic conditions we report a novel phantom of the human prostate that can be resected with TURP. The phantom mirrors the anatomy and haptic properties of the gland and permits quantitative evaluation of important surgical performance indicators. Mixtures of soft materials are engineered to mimic the physical properties of the human tissue, including the mechanical strength, the electrical and thermal conductivity, and the appearance under an endoscope. Electrocautery resection of the phantom closely resembles the procedure on human tissue. Ultrasound contrast agent was applied to the central zone, which was not detectable by the surgeon during the surgery but showed high contrast when imaged after the surgery, to serve as a label for the quantitative evaluation of the surgery. Quantitative criteria for performance assessment are established and evaluated by automated image analysis. We present the workflow of a surgical simulation on a prostate phantom followed by quantitative evaluation of the surgical performance. Surgery on the phantom is useful for medical training, and enables the development and testing of endoscopic and minimally invasive surgical instruments.

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link (url) DOI [BibTex]

link (url) DOI [BibTex]


Interactive Materials – Drivers of Future Robotic Systems
Interactive Materials – Drivers of Future Robotic Systems

Fischer, P.

Adv. Mat., January 2020 (article)

Abstract
A robot senses its environment, processes the sensory information, acts in response to these inputs, and possibly communicates with the outside world. Robots generally achieve these tasks with electronics-based hardware or by receiving inputs from some external hardware. In contrast, simple microorganisms can autonomously perceive, act, and communicate via purely physicochemical processes in soft material systems. A key property of biological systems is that they are built from energy-consuming ‘active’ units. Exciting developments in material science show that even very simple artificial active building blocks can show surprisingly rich emergent behaviors. Active non-equilibrium systems are therefore predicted to play an essential role to realize interactive materials. A major challenge is to find robust ways to couple and integrate the energy-consuming building blocks to the mechanical structure of the material. However, success in this endeavor will lead to a new generation of sophisticated micro- and soft-robotic systems that can operate autonomously.

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link (url) DOI [BibTex]


Thermal Effects on the Crystallization Kinetics, and Interfacial Adhesion of Single-Crystal Phase-Change Gallium
Thermal Effects on the Crystallization Kinetics, and Interfacial Adhesion of Single-Crystal Phase-Change Gallium

Yunusa, M., Lahlou, A., Sitti, M.

Advanced Materials, Wiley Online Library, 2020 (article)

Abstract
Although substrates play an important role upon crystallization of supercooled liquids, the influences of surface temperature and thermal property have remained elusive. Here, the crystallization of supercooled phase‐change gallium (Ga) on substrates with different thermal conductivity is studied. The effect of interfacial temperature on the crystallization kinetics, which dictates thermo‐mechanical stresses between the substrate and the crystallized Ga, is investigated. At an elevated surface temperature, close to the melting point of Ga, an extended single‐crystal growth of Ga on dielectric substrates due to layering effect and annealing is realized without the application of external fields. Adhesive strength at the interfaces depends on the thermal conductivity and initial surface temperature of the substrates. This insight can be applicable to other liquid metals for industrial applications, and sheds more light on phase‐change memory crystallization.

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[BibTex]


Nanoerythrosome-functionalized biohybrid microswimmers
Nanoerythrosome-functionalized biohybrid microswimmers

Buss, N., Yasa, O., Alapan, Y., Akolpoglu, M. B., Sitti, M.

APL Bioengineering, 4, AIP Publishing LLC, 2020 (article)

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[BibTex]

[BibTex]


Injectable Nanoelectrodes Enable Wireless Deep Brain Stimulation of Native Tissue in Freely Moving Mice
Injectable Nanoelectrodes Enable Wireless Deep Brain Stimulation of Native Tissue in Freely Moving Mice

Kozielski, K. L., Jahanshahi, A., Gilbert, H. B., Yu, Y., Erin, O., Francisco, D., Alosaimi, F., Temel, Y., Sitti, M.

bioRxiv, Cold Spring Harbor Laboratory, 2020 (article)

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[BibTex]

[BibTex]


Magnetically Actuated Soft Capsule Endoscope for Fine-Needle Biopsy
Magnetically Actuated Soft Capsule Endoscope for Fine-Needle Biopsy

Son, D., Gilbert, H., Sitti, M.

Soft robotics, Mary Ann Liebert, Inc., publishers 140 Huguenot Street, 3rd Floor New …, 2020 (article)

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[BibTex]

[BibTex]


Mechanical coupling of puller and pusher active microswimmers influences motility
Mechanical coupling of puller and pusher active microswimmers influences motility

Singh, A. V., Kishore, V., Santamauro, G., Yasa, O., Bill, J., Sitti, M.

Langmuir, ACS Publications, 2020 (article)

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[BibTex]


Controlling two-dimensional collective formation and cooperative behavior of magnetic microrobot swarms
Controlling two-dimensional collective formation and cooperative behavior of magnetic microrobot swarms

Dong, X., Sitti, M.

The International Journal of Robotics Research, 2020 (article)

Abstract
Magnetically actuated mobile microrobots can access distant, enclosed, and small spaces, such as inside microfluidic channels and the human body, making them appealing for minimally invasive tasks. Despite their simplicity when scaling down, creating collective microrobots that can work closely and cooperatively, as well as reconfigure their formations for different tasks, would significantly enhance their capabilities such as manipulation of objects. However, a challenge of realizing such cooperative magnetic microrobots is to program and reconfigure their formations and collective motions with under-actuated control signals. This article presents a method of controlling 2D static and time-varying formations among collective self-repelling ferromagnetic microrobots (100 μm to 350 μm in diameter, up to 260 in number) by spatially and temporally programming an external magnetic potential energy distribution at the air–water interface or on solid surfaces. A general design method is introduced to program external magnetic potential energy using ferromagnets. A predictive model of the collective system is also presented to predict the formation and guide the design procedure. With the proposed method, versatile complex static formations are experimentally demonstrated and the programmability and scaling effects of formations are analyzed. We also demonstrate the collective mobility of these magnetic microrobots by controlling them to exhibit bio-inspired collective behaviors such as aggregation, directional motion with arbitrary swarm headings, and rotational swarming motion. Finally, the functions of the produced microrobotic swarm are demonstrated by controlling them to navigate through cluttered environments and complete reconfigurable cooperative manipulation tasks.

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DOI [BibTex]


Magnetic Resonance Imaging System--Driven Medical Robotics
Magnetic Resonance Imaging System–Driven Medical Robotics

Erin, O., Boyvat, M., Tiryaki, M. E., Phelan, M., Sitti, M.

Advanced Intelligent Systems, 2, Wiley Online Library, 2020 (article)

Abstract
Magnetic resonance imaging (MRI) system–driven medical robotics is an emerging field that aims to use clinical MRI systems not only for medical imaging but also for actuation, localization, and control of medical robots. Submillimeter scale resolution of MR images for soft tissues combined with the electromagnetic gradient coil–based magnetic actuation available inside MR scanners can enable theranostic applications of medical robots for precise image‐guided minimally invasive interventions. MRI‐driven robotics typically does not introduce new MRI instrumentation for actuation but instead focuses on converting already available instrumentation for robotic purposes. To use the advantages of this technology, various medical devices such as untethered mobile magnetic robots and tethered active catheters have been designed to be powered magnetically inside MRI systems. Herein, the state‐of‐the‐art progress, challenges, and future directions of MRI‐driven medical robotic systems are reviewed.

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[BibTex]

[BibTex]


Characterization and Thermal Management of a DC Motor-Driven Resonant Actuator for Miniature Mobile Robots with Oscillating Limbs
Characterization and Thermal Management of a DC Motor-Driven Resonant Actuator for Miniature Mobile Robots with Oscillating Limbs

Colmenares, D., Kania, R., Liu, M., Sitti, M.

arXiv preprint arXiv:2002.00798, 2020 (article)

Abstract
In this paper, we characterize the performance of and develop thermal management solutions for a DC motor-driven resonant actuator developed for flapping wing micro air vehicles. The actuator, a DC micro-gearmotor connected in parallel with a torsional spring, drives reciprocal wing motion. Compared to the gearmotor alone, this design increased torque and power density by 161.1% and 666.8%, respectively, while decreasing the drawn current by 25.8%. Characterization of the actuator, isolated from nonlinear aerodynamic loading, results in standard metrics directly comparable to other actuators. The micro-motor, selected for low weight considerations, operates at high power for limited duration due to thermal effects. To predict system performance, a lumped parameter thermal circuit model was developed. Critical model parameters for this micro-motor, two orders of magnitude smaller than those previously characterized, were identified experimentally. This included the effects of variable winding resistance, bushing friction, speed-dependent forced convection, and the addition of a heatsink. The model was then used to determine a safe operation envelope for the vehicle and to design a weight-optimal heatsink. This actuator design and thermal modeling approach could be applied more generally to improve the performance of any miniature mobile robot or device with motor-driven oscillating limbs or loads.

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[BibTex]


Pros and Cons: Magnetic versus Optical Microrobots
Pros and Cons: Magnetic versus Optical Microrobots

Sitti, M., Wiersma, D. S.

Advanced Materials, Wiley Online Library, 2020 (article)

Abstract
Mobile microrobotics has emerged as a new robotics field within the last decade to create untethered tiny robots that can access and operate in unprecedented, dangerous, or hard‐to‐reach small spaces noninvasively toward disruptive medical, biotechnology, desktop manufacturing, environmental remediation, and other potential applications. Magnetic and optical actuation methods are the most widely used actuation methods in mobile microrobotics currently, in addition to acoustic and biological (cell‐driven) actuation approaches. The pros and cons of these actuation methods are reported here, depending on the given context. They can both enable long‐range, fast, and precise actuation of single or a large number of microrobots in diverse environments. Magnetic actuation has unique potential for medical applications of microrobots inside nontransparent tissues at high penetration depths, while optical actuation is suitable for more biotechnology, lab‐/organ‐on‐a‐chip, and desktop manufacturing types of applications with much less surface penetration depth requirements or with transparent environments. Combining both methods in new robot designs can have a strong potential of combining the pros of both methods. There is still much progress needed in both actuation methods to realize the potential disruptive applications of mobile microrobots in real‐world conditions.

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[BibTex]

[BibTex]


Selectively Controlled Magnetic Microrobots with Opposing Helices
Selectively Controlled Magnetic Microrobots with Opposing Helices

Giltinan, J., Katsamba, P., Wang, W., Lauga, E., Sitti, M.

Applied Physics Letters, 116, AIP Publishing LLC, 2020 (article)

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[BibTex]

[BibTex]


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Microscale Polarization Color Pixels from Liquid Crystal Elastomers

Yubing, , Hamed, , Metin,

Advanced Optical Materials, 2020 (article) Accepted

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[BibTex]

[BibTex]


Cohesive self-organization of mobile microrobotic swarms
Cohesive self-organization of mobile microrobotic swarms

Yigit, B., Alapan, Y., Sitti, M.

arXiv preprint arXiv:1907.05856, 2020 (article)

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[BibTex]

[BibTex]


Bio-inspired Flexible Twisting Wings Increase Lift and Efficiency of a Flapping Wing Micro Air Vehicle
Bio-inspired Flexible Twisting Wings Increase Lift and Efficiency of a Flapping Wing Micro Air Vehicle

Colmenares, D., Kania, R., Zhang, W., Sitti, M.

arXiv preprint arXiv:2001.11586, 2020 (article)

Abstract
We investigate the effect of wing twist flexibility on lift and efficiency of a flapping-wing micro air vehicle capable of liftoff. Wings used previously were chosen to be fully rigid due to modeling and fabrication constraints. However, biological wings are highly flexible and other micro air vehicles have successfully utilized flexible wing structures for specialized tasks. The goal of our study is to determine if dynamic twisting of flexible wings can increase overall aerodynamic lift and efficiency. A flexible twisting wing design was found to increase aerodynamic efficiency by 41.3%, translational lift production by 35.3%, and the effective lift coefficient by 63.7% compared to the rigid-wing design. These results exceed the predictions of quasi-steady blade element models, indicating the need for unsteady computational fluid dynamics simulations of twisted flapping wings.

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[BibTex]

[BibTex]


Acoustically powered surface-slipping mobile microrobots
Acoustically powered surface-slipping mobile microrobots

Aghakhani, A., Yasa, O., Wrede, P., Sitti, M.

Proceedings of the National Academy of Sciences, 117, National Acad Sciences, 2020 (article)

Abstract
Untethered synthetic microrobots have significant potential to revolutionize minimally invasive medical interventions in the future. However, their relatively slow speed and low controllability near surfaces typically are some of the barriers standing in the way of their medical applications. Here, we introduce acoustically powered microrobots with a fast, unidirectional surface-slipping locomotion on both flat and curved surfaces. The proposed three-dimensionally printed, bullet-shaped microrobot contains a spherical air bubble trapped inside its internal body cavity, where the bubble is resonated using acoustic waves. The net fluidic flow due to the bubble oscillation orients the microrobot's axisymmetric axis perpendicular to the wall and then propels it laterally at very high speeds (up to 90 body lengths per second with a body length of 25 µm) while inducing an attractive force toward the wall. To achieve unidirectional locomotion, a small fin is added to the microrobot’s cylindrical body surface, which biases the propulsion direction. For motion direction control, the microrobots are coated anisotropically with a soft magnetic nanofilm layer, allowing steering under a uniform magnetic field. Finally, surface locomotion capability of the microrobots is demonstrated inside a three-dimensional circular cross-sectional microchannel under acoustic actuation. Overall, the combination of acoustic powering and magnetic steering can be effectively utilized to actuate and navigate these microrobots in confined and hard-to-reach body location areas in a minimally invasive fashion.

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[BibTex]

[BibTex]


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Morphology-Dependent Immunogenicity Obliges a Compromise on the Locomotion-Focused Design of Medical Microrobots

Ceren, , Hakan, , Ugur, , Anna-Maria, , Metin,

Science Robotics, 2020 (article) Accepted

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[BibTex]

[BibTex]


Bioinspired underwater locomotion of light-driven liquid crystal gels
Bioinspired underwater locomotion of light-driven liquid crystal gels

Shahsavan, H., Aghakhani, A., Zeng, H., Guo, Y., Davidson, Z. S., Priimagi, A., Sitti, M.

Proceedings of the National Academy of Sciences, National Acad Sciences, 2020 (article)

Abstract
Untethered dynamic shape programming and control of soft materials have significant applications in technologies such as soft robots, medical devices, organ-on-a-chip, and optical devices. Here, we present a solution to remotely actuate and move soft materials underwater in a fast, efficient, and controlled manner using photoresponsive liquid crystal gels (LCGs). LCG constructs with engineered molecular alignment show a low and sharp phase-transition temperature and experience considerable density reduction by light exposure, thereby allowing rapid and reversible shape changes. We demonstrate different modes of underwater locomotion, such as crawling, walking, jumping, and swimming, by localized and time-varying illumination of LCGs. The diverse locomotion modes of smart LCGs can provide a new toolbox for designing efficient light-fueled soft robots in fluid-immersed media.

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[BibTex]

[BibTex]


Additive manufacturing of cellulose-based materials with continuous, multidirectional stiffness gradients
Additive manufacturing of cellulose-based materials with continuous, multidirectional stiffness gradients

Giachini, P., Gupta, S., Wang, W., Wood, D., Yunusa, M., Baharlou, E., Sitti, M., Menges, A.

Science Advances, 6, American Association for the Advancement of Science, 2020 (article)

Abstract
Functionally graded materials (FGMs) enable applications in fields such as biomedicine and architecture, but their fabrication suffers from shortcomings in gradient continuity, interfacial bonding, and directional freedom. In addition, most commercial design software fail to incorporate property gradient data, hindering explorations of the design space of FGMs. Here, we leveraged a combined approach of materials engineering and digital processing to enable extrusion-based multimaterial additive manufacturing of cellulose-based tunable viscoelastic materials with continuous, high-contrast, and multidirectional stiffness gradients. A method to engineer sets of cellulose-based materials with similar compositions, yet distinct mechanical and rheological properties, was established. In parallel, a digital workflow was developed to embed gradient information into design models with integrated fabrication path planning. The payoff of integrating these physical and digital tools is the ability to achieve the same stiffness gradient in multiple ways, opening design possibilities previously limited by the rigid coupling of material and geometry.

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[BibTex]

[BibTex]


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Introducing Progress in Biomedical Engineering; Issue 2 Vol 2

Sitti, M.

Progress in Biomedical Engineering, IOP Publishing, 2020 (article)

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[BibTex]

[BibTex]


Multi-wavelength steerable visible light-driven magnetic CoO-TiO2 microswimmers
Multi-wavelength steerable visible light-driven magnetic CoO-TiO2 microswimmers

Sridhar, V., Park, B., Guo, S., van Aken, P. A., Sitti, M.

ACS Applied Materials \& Interfaces, ACS Publications, 2020 (article)

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[BibTex]

[BibTex]

2005


Nonlinear optical spectroscopy of chiral molecules
Nonlinear optical spectroscopy of chiral molecules

Fischer, P., Hache, F.

CHIRALITY, 17(8):421-437, 2005 (article)

Abstract
We review nonlinear optical processes that are specific to chiral molecules in solution and on surfaces. In contrast to conventional natural optical activity phenomena, which depend linearly on the electric field strength of the optical field, we discuss how optical processes that are nonlinear (quadratic, cubic, and quartic) functions of the electromagnetic field strength may probe optically active centers and chiral vibrations. We show that nonlinear techniques open entirely new ways of exploring chirality in chemical and biological systems: The cubic processes give rise to nonlinear circular dichroism and nonlinear optical rotation and make it possible to observe dynamic chiral processes at ultrafast time scales. The quadratic second-harmonic and sum-frequency-generation phenomena and the quartic processes may arise entirely in the electric-dipole approximation and do not require the use of circularly polarized light to detect chirality: They provide surface selectivity and their observables can be relatively much larger than in linear optical activity. These processes also give rise to the generation of light at a new color, and in liquids this frequency conversion only occurs if the solution is optically active. We survey recent chiral nonlinear optical experiments and give examples of their application to problems of biophysical interest. (C) 2005 Wiley-Liss, Inc.

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DOI [BibTex]

2005


DOI [BibTex]


Negative refraction at optical frequencies in nonmagnetic two-component molecular media
Negative refraction at optical frequencies in nonmagnetic two-component molecular media

Chen, Y., Fischer, P., Wise, F.

PHYSICAL REVIEW LETTERS, 95(6), 2005 (article)

Abstract
There is significant motivation to develop media with negative refractive indices at optical frequencies, but efforts in this direction are hampered by the weakness of the magnetic response at such frequencies. We show theoretically that a nonmagnetic medium with two atomic or molecular constituents can exhibit a negative refractive index. A negative index is possible even when the real parts of both the permittivity and permeability are positive. This surprising result provides a route to isotropic negative-index media at optical frequencies.

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DOI [BibTex]

DOI [BibTex]


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Modeling and testing of a biomimetic flagellar propulsion method for microscale biomedical swimming robots

Behkam, B., Sitti, M.

In Proceedings of Advanced Intelligent Mechatronics Conference, pages: 37-42, 2005 (inproceedings)

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Project Page [BibTex]

Project Page [BibTex]


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Biologically inspired adhesion based surface climbing robots

Menon, C., Sitti, M.

In Robotics and Automation, 2005. ICRA 2005. Proceedings of the 2005 IEEE International Conference on, pages: 2715-2720, 2005 (inproceedings)

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[BibTex]

[BibTex]


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Claytronics: highly scalable communications, sensing, and actuation networks

Aksak, Burak, Bhat, Preethi Srinivas, Campbell, Jason, DeRosa, Michael, Funiak, Stanislav, Gibbons, Phillip B, Goldstein, Seth Copen, Guestrin, Carlos, Gupta, Ashish, Helfrich, Casey, others

In Proceedings of the 3rd international conference on Embedded networked sensor systems, pages: 299-299, 2005 (inproceedings)

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[BibTex]

[BibTex]


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Biologically Inspired Miniature Water Strider Robot.

Suhr, S. H., Song, Y. S., Lee, S. J., Sitti, M.

In Robotics: Science and Systems, pages: 319-326, 2005 (inproceedings)

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[BibTex]

[BibTex]


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Polymer micro/nanofiber fabrication using micro/nanopipettes

Nain, A. S., Amon, C., Sitti, M.

In Nanotechnology, 2005. 5th IEEE Conference on, pages: 366-369, 2005 (inproceedings)

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[BibTex]

[BibTex]


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Fusion of biomedical microcapsule endoscope and microsystem technology

Kim, Tae Song, Kim, Byungkyu, Cho, Dongil Dan, Song, Si Young, Dario, P, Sitti, M

In Solid-State Sensors, Actuators and Microsystems, 2005. Digest of Technical Papers. TRANSDUCERS’05. The 13th International Conference on, 1, pages: 9-14, 2005 (inproceedings)

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[BibTex]


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Atomic force microscope based two-dimensional assembly of micro/nanoparticles

Tafazzoli, A., Pawashe, C., Sitti, M.

In Assembly and Task Planning: From Nano to Macro Assembly and Manufacturing, 2005.(ISATP 2005). The 6th IEEE International Symposium on, pages: 230-235, 2005 (inproceedings)

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[BibTex]


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A new endoscopic microcapsule robot using beetle inspired microfibrillar adhesives

Cheung, E., Karagozler, M. E., Park, S., Kim, B., Sitti, M.

In Advanced Intelligent Mechatronics. Proceedings, 2005 IEEE/ASME International Conference on, pages: 551-557, 2005 (inproceedings)

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Project Page [BibTex]

Project Page [BibTex]

2001


Isotropic second-order nonlinear optical susceptibilities
Isotropic second-order nonlinear optical susceptibilities

Fischer, P., Buckingham, A., Albrecht, A.

PHYSICAL REVIEW A, 64(5), 2001 (article)

Abstract
The second-order nonlinear optical susceptibility, in the electric dipole approximation, is only nonvanishing for materials that are noncentrosymmetric. Should the medium be isotropic, then only a chiral system. such as an optically active liquid, satisfies this symmetry requirement. We derive the quantum-mechanical form of the isotropic component of the sum- and difference-frequency susceptibility and discuss its unusual spectral properties. We show that any coherent second-order nonlinear optical process in a system of randomly oriented molecules requires the medium to be chiral. and the incident frequencies to be different and nonzero. Furthermore, a minimum of two nondegenerate excited molecular states are needed for the isotropic part of the susceptibility to be nonvanishing. The rotationally invariant susceptibility is zero in the static field limit and shows exceptionally sensitive resonance and dephasing effects that are particular to chiral centers.

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DOI [BibTex]

2001


DOI [BibTex]


Reply to ``Comment on `Phenomenological damping in optical response tensors'{''}
Reply to “Comment on ‘Phenomenological damping in optical response tensors’”

Buckingham, A., Fischer, P.

PHYSICAL REVIEW A, 63(4), 2001 (article)

Abstract
We show that damping factors must not be incorporated in the perturbation of the ground state by a static electric field. If they are included, as in the theory of Stedman et al. {[}preceding Comment. Phys. Rev. A 63, 047801 (2001)], then there would be an electric dipole in the y direction induced in a hydrogen atom in the M-s = + 1/2 state by a static electric field in the x direction. Such a dipole is excluded by symmetry.

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DOI [BibTex]


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Survey of nanomanipulation systems

Sitti, M.

In Nanotechnology, 2001. IEEE-NANO 2001. Proceedings of the 2001 1st IEEE Conference on, pages: 75-80, 2001 (inproceedings)

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[BibTex]

[BibTex]


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Nanotribological characterization system by AFM based controlled pushing

Sitti, M.

In Nanotechnology, 2001. IEEE-NANO 2001. Proceedings of the 2001 1st IEEE Conference on, pages: 99-104, 2001 (inproceedings)

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[BibTex]

[BibTex]


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Towards flapping wing control for a micromechanical flying insect

Yan, J., Wood, R. J., Avadhanula, S., Sitti, M., Fearing, R. S.

In Robotics and Automation, 2001. Proceedings 2001 ICRA. IEEE International Conference on, 4, pages: 3901-3908, 2001 (inproceedings)

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[BibTex]


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Man-machine interface for micro/nano manipulation with an afm probe

Aruk, B., Hashimoto, H., Sitti, M.

In Nanotechnology, 2001. IEEE-NANO 2001. Proceedings of the 2001 1st IEEE Conference on, pages: 151-156, 2001 (inproceedings)

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Development of PZT and PZN-PT based unimorph actuators for micromechanical flapping mechanisms

Sitti, M., Campolo, D., Yan, J., Fearing, R. S.

In Robotics and Automation, 2001. Proceedings 2001 ICRA. IEEE International Conference on, 4, pages: 3839-3846, 2001 (inproceedings)

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Thorax Design and Wing Control for a Micromechanical Flying Insect

Yan, J, Ayadhanula, S, Sitti, M, Wood, RJ, Fearing, RS

In PROCEEDINGS OF THE ANNUAL ALLERTON CONFERENCE ON COMMUNICATION CONTROL AND COMPUTING, 39(2):952-961, 2001 (inproceedings)

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PZT actuated four-bar mechanism with two flexible links for micromechanical flying insect thorax

Sitti, M.

In Robotics and Automation, 2001. Proceedings 2001 ICRA. IEEE International Conference on, 4, pages: 3893-3900, 2001 (inproceedings)

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Wing transmission for a micromechanical flying insect

Yan, J., Avadhanula, S., Birch, J., Dickinson, M., Sitti, M., Su, T., Fearing, R.

Journal of Micromechatronics, 1(3):221-237, Brill, 2001 (article)

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Development of a scaled teleoperation system for nano scale interaction and manipulation

Sitti, M., Aruk, B., Shintani, H., Hashimoto, H.

In Robotics and Automation, 2001. Proceedings 2001 ICRA. IEEE International Conference on, 1, pages: 860-867, 2001 (inproceedings)

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[BibTex]

[BibTex]